Regulating Photocatalytic CO2 Reduction Kinetics through Modification of Surface Coordination Sphere

C Feng, T Bo, P Maity, S Zuo, W Zhou… - Advanced Functional …, 2024 - Wiley Online Library
Solar‐driven reduction of CO2 to value‐added products represents a sustainable strategy
for mitigating the greenhouse effect and addressing the related green‐energy crisis. Herein …

Ultrafast relaxation of lattice distortion in two-dimensional perovskites

H Zhang, W Li, J Essman, C Quarti, I Metcalf… - Nature Physics, 2023 - nature.com
Direct visualization of ultrafast coupling between charge carriers and lattice degrees of
freedom in photoexcited semiconductors has remained a long-standing challenge and is …

Enhancing the hot carrier injection of perovskite solar cells by incorporating a molecular dipole interlayer

T Wu, R Zhao, J Qiu, S Wang… - Advanced Functional …, 2022 - Wiley Online Library
Surface passivation engineering of perovskite films via organic functional small molecules
has emerged as an effective strategy for improving the efficiency and stability of perovskite …

Multiple exciton generation in tin–lead halide perovskite nanocrystals for photocurrent quantum efficiency enhancement

Y Chen, J Yin, Q Wei, C Wang, X Wang, H Ren… - Nature …, 2022 - nature.com
Multiple exciton generation (MEG), the generation of multiple electron–hole pairs from a
single high-energy photon, can enhance the photoconversion efficiency in several …

Long-Lived Hot Carriers in Two-Dimensional Perovskites: The Role of Alternating Cations in Interlayer Space

Q Wei, H Ren, J Liu, Q Liu, C Wang, TW Lau… - ACS Energy …, 2023 - ACS Publications
Solar absorbers featuring prolonged hot-carrier (HC) cooling are highly desired for the
development of HC solar cells. Two-dimensional (2D) hybrid perovskites are known for their …

Control of hot carrier cooling in lead halide perovskites by point defects

Z Zhou, J He, T Frauenheim, OV Prezhdo… - Journal of the …, 2022 - ACS Publications
Hot carriers (HCs) in lead halide perovskites are prone to rapidly relax at the band edge and
waste plentiful photon energy, severely limiting their conversion efficiency as HC …

Moisture‐Tailored 2D Dion–Jacobson Perovskites for Reconfigurable Optoelectronics

M Guan, Y **e, Y Zhang, Z Gu, L Qiu, Z He… - Advanced …, 2023 - Wiley Online Library
Humidity‐and moisture‐induced degradation has been a longstanding problem in
perovskite materials, affecting their long‐term stability during applications. Counterintuitively …

Thermalization and relaxation mediated by phonon management in tin-lead perovskites

L Dai, J Ye, NC Greenham - Light: Science & Applications, 2023 - nature.com
Understanding and control of ultrafast non-equilibrium processes in semiconductors is key
to making use of the full photon energy before relaxation, leading to new ways to break …

Spin–orbit coupling in 2D semiconductors: A theoretical perspective

J Chen, K Wu, W Hu, J Yang - The Journal of Physical Chemistry …, 2021 - ACS Publications
This theoretical Perspective reviews spin–orbit coupling (SOC), including the Rashba effect
and Dresselhaus effect, in two-dimensional (2D) semiconductors. We first introduce the …

Hot-carrier tunable abnormal nonlinear absorption conversion in quasi-2D perovskite

G Wang, T Liu, B Wang, H Gu, Q Wei, Z Zhang… - Nature …, 2022 - nature.com
Controlling the high-power laser transmittance is built on the diverse manipulation of
multiple nonlinear absorption (NLA) processes in the nonlinear optical (NLO) materials …