Spatially and temporally understanding dynamic solid–electrolyte interfaces in carbon dioxide electroreduction

J Wang, HY Tan, MY Qi, JY Li, ZR Tang… - Chemical Society …, 2023 - pubs.rsc.org
The ubiquity of solid–liquid interfaces in nature and the significant role of their atomic-scale
structure in determining interfacial properties have led to intensive research. Particularly in …

Comprehensive understandings into complete reconstruction of precatalysts: synthesis, applications, and characterizations

X Liu, J Meng, J Zhu, M Huang, B Wen… - Advanced …, 2021 - Wiley Online Library
Reconstruction induced by external environment (such as applied voltage bias and test
electrolytes) changes catalyst component and catalytic behaviors. Investigations of complete …

In Situ Infrared Spectroscopic Evidence of Enhanced Electrochemical CO2 Reduction and C–C Coupling on Oxide-Derived Copper

EP Delmo, Y Wang, Y Song, S Zhu… - Journal of the …, 2024 - ACS Publications
The reaction mechanism of CO2 electroreduction on oxide-derived copper has not yet been
unraveled even though high C2+ Faradaic efficiencies are commonly observed on these …

Chemical and Structural Evolution of AgCu Catalysts in Electrochemical CO2 Reduction

PC Chen, C Chen, Y Yang, AL Maulana… - Journal of the …, 2023 - ACS Publications
Silver–copper (AgCu) bimetallic catalysts hold great potential for electrochemical carbon
dioxide reduction reaction (CO2RR), which is a promising way to realize the goal of carbon …

In situ X-ray spectroscopies beyond conventional X-ray absorption spectroscopy on deciphering dynamic configuration of electrocatalysts

J Wang, CS Hsu, TS Wu, TS Chan, NT Suen… - Nature …, 2023 - nature.com
Realizing viable electrocatalytic processes for energy conversion/storage strongly relies on
an atomic-level understanding of dynamic configurations on catalyst-electrolyte interface. X …

Modeling Operando Electrochemical CO2 Reduction

F Dattila, RR Seemakurthi, Y Zhou, N López - Chemical Reviews, 2022 - ACS Publications
Since the seminal works on the application of density functional theory and the
computational hydrogen electrode to electrochemical CO2 reduction (eCO2R) and …

Linking the Dynamic Chemical State of Catalysts with the Product Profile of Electrocatalytic CO2 Reduction

J Wang, HY Tan, Y Zhu, H Chu… - Angewandte Chemie, 2021 - Wiley Online Library
The promoted activity and enhanced selectivity of electrocatalysts is commonly ascribed to
specific structural features such as surface facets, morphology, and atomic defects …

Progress and Perspectives of Electrochemical CO2 Reduction on Copper in Aqueous Electrolyte

S Nitopi, E Bertheussen, SB Scott, X Liu… - Chemical …, 2019 - ACS Publications
To date, copper is the only heterogeneous catalyst that has shown a propensity to produce
valuable hydrocarbons and alcohols, such as ethylene and ethanol, from electrochemical …

Emerging dynamic structure of electrocatalysts unveiled by in situ X-ray diffraction/absorption spectroscopy

Y Zhu, TR Kuo, YH Li, MY Qi, G Chen… - Energy & …, 2021 - pubs.rsc.org
Highly-efficient oxygen evolution reaction (OER) and reduction of carbon dioxide (CO2RR)
represent the two biggest scientific challenges in artificial photosynthesis. Many efficient and …

Designing copper‐based catalysts for efficient carbon dioxide electroreduction

Y Wang, J Liu, G Zheng - Advanced Materials, 2021 - Wiley Online Library
The electroreduction of carbon dioxide (CO2) has been emerging as a high‐potential
approach for CO2 utilization using renewables. When copper (Cu) based catalysts are used …