Deep-ultraviolet nonlinear optical crystals: concept development and materials discovery

L Kang, Z Lin - Light: Science & Applications, 2022 - nature.com
Deep-ultraviolet (DUV, wavelength λ< 200 nm) nonlinear optical (NLO) crystal is the core
component of frequency conversion to generate DUV laser, which plays an important role in …

New Functional Groups Design toward High Performance Ultraviolet Nonlinear Optical Materials

H Fan, N Ye, M Luo - Accounts of Chemical Research, 2023 - ACS Publications
Conspectus The invention of the laser is a pivotal milestone in the evolution of modern
science and technology. Second-order nonlinear optical (NLO) crystals, which possess the …

Finding the Next Deep-Ultraviolet Nonlinear Optical Material: NH4B4O6F

G Shi, Y Wang, F Zhang, B Zhang, Z Yang… - Journal of the …, 2017 - ACS Publications
Nonlinear optical materials are essential for the development of solid-state lasers.
KBe2BO3F2 (KBBF) is a unique nonlinear optical material for generation of deep-ultraviolet …

Large Second-Harmonic Response and Giant Birefringence of CeF2(SO4) Induced by Highly Polarizable Polyhedra

C Wu, T Wu, X Jiang, Z Wang, H Sha… - Journal of the …, 2021 - ACS Publications
Second-harmonic generation (SHG) response and birefringence are two critically important
properties of nonlinear optical (NLO) materials. However, the simultaneous optimization of …

K2Sb(P2O7)F: Cairo Pentagonal Layer with Bifunctional Genes Reveal Optical Performance

Y Deng, L Huang, X Dong, L Wang… - Angewandte Chemie …, 2020 - Wiley Online Library
Discovering new functional genes, designing perfect crystal structures, and develo** high‐
performance materials are the goals being pursued by scientists. Herein, the first antimony …

CsSbF2SO4: An Excellent Ultraviolet Nonlinear Optical Sulfate with a KTiOPO4 (KTP)‐type Structure

X Dong, L Huang, C Hu, H Zeng, Z Lin… - Angewandte …, 2019 - Wiley Online Library
A novel noncentrosymmetric (NCS) polar fluoride sulfate, CsSbF2SO4, was obtained by
ionothermal synthesis. A meticulously designed co‐substitution approach was used to …

Novel ultraviolet (UV) nonlinear optical (NLO) materials discovered by chemical substitution-oriented design

G Zou, KM Ok - Chemical Science, 2020 - pubs.rsc.org
Exploring novel functional materials via chemical substitution-oriented design is an
emerging strategy. The method can be expanded to the discovery of high performance …

Emergent deep‐ultraviolet nonlinear optical candidates

M Mutailipu, S Pan - Angewandte Chemie International Edition, 2020 - Wiley Online Library
Advances in the generation of coherent lasers at wavelengths below 200 nm as well as the
associated equipment and technologies have greatly spurred the development of nonlinear …

Giant Optical Anisotropy in the UV‐Transparent 2D Nonlinear Optical Material Sc(IO3)2(NO3)

C Wu, X Jiang, Z Wang, L Lin, Z Lin… - Angewandte …, 2021 - Wiley Online Library
Birefringence is a fundamental optical property for linear and nonlinear optical (NLO)
materials. Thus far, it has proved to be very difficult to engineer large birefringence in optical …

Exploring Short-Wavelength Phase-Matching Nonlinear Optical Crystals by Employing KBe2BO3F2 as the Template

Z Li, W **, F Zhang, Z Yang, S Pan - ACS Central Science, 2022 - ACS Publications
Exploration of nonlinear optical (NLO) crystals that are competent in generating short-
wavelength ultraviolet (UV, λ≤ 266 nm, and even deep-UV, λ≤ 200 nm) coherent light …