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Direct laser cooling of polyatomic molecules
Over the past decade, tremendous progress has been made to extend the tools of laser
cooling and trap** to molecules. Those same tools have recently been applied to …
cooling and trap** to molecules. Those same tools have recently been applied to …
Magneto-optical trap** and sub-Doppler cooling of a polyatomic molecule
Laser cooling and trap**,, and magneto-optical trap** methods in particular, have
enabled groundbreaking advances in science, including Bose–Einstein condensation …
enabled groundbreaking advances in science, including Bose–Einstein condensation …
An optical tweezer array of ultracold polyatomic molecules
Polyatomic molecules have rich structural features that make them uniquely suited to
applications in quantum information science,–, quantum simulation,–, ultracold chemistry …
applications in quantum information science,–, quantum simulation,–, ultracold chemistry …
Optical Trap** of a Polyatomic Molecule in an -Type Parity Doublet State
We report optical trap** of a polyatomic molecule, calcium monohydroxide (CaOH). CaOH
molecules from a magneto-optical trap are sub-Doppler laser cooled to 20 (3) μ K in free …
molecules from a magneto-optical trap are sub-Doppler laser cooled to 20 (3) μ K in free …
Functionalizing aromatic compounds with optical cycling centres
Molecular design principles provide guidelines for augmenting a molecule with a smaller
group of atoms to realize a desired property or function. We demonstrate that these concepts …
group of atoms to realize a desired property or function. We demonstrate that these concepts …
Absolute frequency metrology of buffer-gas-cooled molecular spectra at 1 kHz accuracy level
By reducing both the internal and translational temperature of any species down to a few
kelvins, the buffer-gas-cooling (BGC) technique has the potential to dramatically improve the …
kelvins, the buffer-gas-cooling (BGC) technique has the potential to dramatically improve the …
Characterizing the fundamental bending vibration of a linear polyatomic molecule for symmetry violation searches
Polyatomic molecules have been identified as sensitive probes of charge-parity violating
and parity violating physics beyond the Standard Model (BSM). For example, many linear …
and parity violating physics beyond the Standard Model (BSM). For example, many linear …
Intensity-borrowing mechanisms pertinent to laser cooling of linear polyatomic molecules
A study of the intensity-borrowing mechanisms important to optical cycling transitions in
laser-coolable polyatomic molecules arising from non-adiabatic coupling, contributions …
laser-coolable polyatomic molecules arising from non-adiabatic coupling, contributions …
Zeeman-Sisyphus deceleration of molecular beams
We present a robust, continuous molecular decelerator that employs high magnetic fields
and few optical pum** steps. CaOH molecules are slowed, accumulating at low velocities …
and few optical pum** steps. CaOH molecules are slowed, accumulating at low velocities …
Optical cycling in polyatomic molecules with complex hyperfine structure
We have developed and demonstrated a scheme to achieve rotationally closed photon
cycling in polyatomic molecules with complex hyperfine structure and sensitivity to hadronic …
cycling in polyatomic molecules with complex hyperfine structure and sensitivity to hadronic …