Reactivity of metal–oxo clusters towards biomolecules: from discrete polyoxometalates to metal–organic frameworks

DES Marcano, ND Savić, K Declerck… - Chemical Society …, 2024 - pubs.rsc.org
Metal–oxo clusters hold great potential in several fields such as catalysis, materials science,
energy storage, medicine, and biotechnology. These nanoclusters of transition metals with …

Exploiting interactions between polyoxometalates and proteins for applications in (bio) chemistry and medicine

S Lentink, DE Salazar Marcano… - Angewandte …, 2023 - Wiley Online Library
The specific interactions of anionic metal‐oxo clusters, known as polyoxometalates (POMs),
with proteins can be leveraged for a wide range of analytical and biomedical applications …

The novel application of polyoxometalates for achieving sludge deep dewatering using low-temperature thermal hydrolysis pretreatment

X Ling, H Zheng, J Huang, H Sun, S Xu, H Zeng… - Journal of Cleaner …, 2024 - Elsevier
Traditional thermal hydrolysis pretreatment (THP) for sludge deep dewatering is energy-
intensive and poses the risk of generating bio-toxic substances that affect downstream …

Speciation atlas of polyoxometalates in aqueous solutions

NI Gumerova, A Rompel - Science Advances, 2023 - science.org
Speciation is the key parameter in solution chemistry that describes the composition,
concentration, and oxidation state of each chemical form of an element present in a sample …

All‐Inorganic Polyoxometalates Act as Superchaotropic Membrane Carriers

A Barba‐Bon, NI Gumerova, E Tanuhadi… - Advanced …, 2024 - Wiley Online Library
Polyoxometalates (POMs) are known antitumoral, antibacterial, antiviral, and anticancer
agents and considered as next‐generation metallodrugs. Herein, a new biological …

Solution-processed formation of DNA-origami-supported polyoxometalate multi-level switches with countercation-controlled conductance tunability

E Vogelsberg, M Moors, AS Sorokina… - Chemistry of …, 2023 - ACS Publications
We report a chemically programmed design and the switching characteristics of a functional
metal–DNA-origami–polyoxometalate (POM) material obtained from the solution-processed …

Effect of the Polyanion Structure on the Mechanism of Alcohol Oxidation with H2O2 Catalyzed by Zr-Substituted Polyoxotungstates

NV Maksimchuk, SM Marikovskaya… - Inorganic …, 2024 - ACS Publications
Zr-monosubstituted polyoxometalates (Zr-POMs) of the Lindqvist (Bu4N) 6 [{W5O18Zr (μ-
OH)} 2](1), Keggin (Bu4N) 8 [{PW11O39Zr (μ-OH)} 2](2), and Wells–Dawson (Bu4N) 11.3 …

Hybrid functional materials merging polyoxometalates and biomolecules: From synthesis to applications

DES Marcano, TN Parac-Vogt - Coordination Chemistry Reviews, 2024 - Elsevier
Recent developments in synthetic strategies have enabled the formation of increasingly
complex hybrid functional materials incorporating both organic and inorganic components …

Polyoxometalates: metallodrug agents for combating amyloid aggregation

M Ma, Z Liu, H Zhao, H Zhang, J Ren… - National Science …, 2024 - academic.oup.com
Alzheimer's disease (AD) is a devastating neurodegenerative disease that affects∼ 50
million people globally. The accumulation of amyloid-β (Aβ) plaques, a predominant …

Tuning Reactivity of Zr-Substituted Keggin Phosphotungstate in Alkene Epoxidation through Balancing H2O2 Activation Pathways: Unusual Effect of Base

NV Maksimchuk, SM Marikovskaya… - Inorganic …, 2023 - ACS Publications
The Zr-monosubstituted Keggin-type dimeric phosphotungstate (Bu4N) 8 [{PW11O39Zr (μ–
OH)(H2O)} 2](1) efficiently catalyzes epoxidation of C═ C bonds in various kinds of alkenes …