Design principles for strong and tough hydrogels

X Li, JP Gong - Nature Reviews Materials, 2024‏ - nature.com
Hydrogels are crosslinked polymer networks swollen with water. Owing to their soft and
water-containing nature, hydrogels are promising materials for applications in many fields …

Dynamic bonds: adaptable timescales for responsive materials

SV Wanasinghe, OJ Dodo… - Angewandte Chemie, 2022‏ - Wiley Online Library
Dynamic bonds introduce unique properties such as self‐healing, recyclability, shape
memory, and malleability to polymers. Significant efforts have been made to synthesize a …

Strong, tough, rapid-recovery, and fatigue-resistant hydrogels made of picot peptide fibres

B Xue, Z Bashir, Y Guo, W Yu, W Sun, Y Li… - Nature …, 2023‏ - nature.com
Hydrogels are promising soft materials as tissue engineering scaffolds, stretchable sensors,
and soft robotics. Yet, it remains challenging to develop synthetic hydrogels with mechanical …

Mechanical Regulation of Polymer Gels

C Xu, Y Chen, S Zhao, D Li, X Tang, H Zhang… - Chemical …, 2024‏ - ACS Publications
The mechanical properties of polymer gels devote to emerging devices and machines in
fields such as biomedical engineering, flexible bioelectronics, biomimetic actuators, and …

Piezoionic Elastomers by Phase and Interface Engineering for High‐Performance Energy‐Harvesting Ionotronics

W Zhu, B Wu, Z Lei, P Wu - Advanced Materials, 2024‏ - Wiley Online Library
Piezoionic materials play a pivotal role in energy‐harvesting ionotronics. However, a
persistent challenge lies in balancing the structural requirements for voltage generation …

Time-salt type superposition and salt processing of poly (methacrylamide) hydrogel based on hofmeister series

Y **, S Lu, X Chen, Q Fang, X Guan, L Qin… - …, 2024‏ - ACS Publications
Breakthrough to the extreme properties of polymer networks relies on new insights into their
molecular dynamics. Time-salt concentration superposition has been discovered in …

Bilayer hydrogels with low friction and high load-bearing capacity by mimicking the oriented hierarchical structure of cartilage

Q Chen, X Zhang, K Chen, C Feng… - … Applied Materials & …, 2022‏ - ACS Publications
Natural articular cartilages exhibit extraordinary lubricating properties and excellent load-
bearing capacity based on their penetrated surface lubricated biomacromolecules and …

Role of hierarchy structure on the mechanical adaptation of self-healing hydrogels under cyclic stretching

X Li, K Cui, Y Zheng, YN Ye, C Yu, W Yang… - Science …, 2023‏ - science.org
Soft materials with mechanical adaptability have substantial potential for various
applications in tissue engineering. Gaining a deep understanding of the structural evolution …

Strain-stiffening, self-healing, and low-hysteresis physically dual-cross-linked hydrogels derived from two mechanically distinct hydrogen bonds

X Yu, Y Wang, H Zhang, Z Li, Y Zheng, X Fan… - Chemistry of …, 2023‏ - ACS Publications
Herein, we propose a facile strategy to fabricate high-performance hydrogels combining
strain-stiffening mechanical behavior with self-healing ability and low hysteresis, which …

Tough hydrogels with different toughening mechanisms and applications

Z Xu, Y Chen, Y Cao, B Xue - International Journal of Molecular Sciences, 2024‏ - mdpi.com
Load-bearing biological tissues, such as cartilage and muscles, exhibit several crucial
properties, including high elasticity, strength, and recoverability. These characteristics …