Coherent multidimensional optical spectroscopy of excitons in molecular aggregates; quasiparticle versus supermolecule perspectives

D Abramavicius, B Palmieri, DV Voronine… - Chemical …, 2009 - ACS Publications
Molecular aggregates are abundant in nature; they form spontaneously in concentrated
solutions and on surfaces and can be synthesized by supramolecular chemistry techniques …

Nonlinear optical signals and spectroscopy with quantum light

KE Dorfman, F Schlawin, S Mukamel - Reviews of Modern Physics, 2016 - APS
Conventional nonlinear spectroscopy uses classical light to detect matter properties through
the variation of its response with frequencies or time delays. Quantum light opens up new …

Symmetry-breaking-induced nonlinear optics at a microcavity surface

X Zhang, QT Cao, Z Wang, Y Liu, CW Qiu, L Yang… - Nature …, 2019 - nature.com
Second-order nonlinear optical processes lie at the heart of many applications in both
classical and quantum regimes,–. Inversion symmetry, however, rules out the second-order …

Nonlinear helical dichroism in chiral and achiral molecules

JL Bégin, A Jain, A Parks, F Hufnagel, P Corkum… - Nature …, 2023 - nature.com
Chiral interactions are prevalent in nature, driving a variety of biochemical processes.
Discerning the two non-superimposable mirror images of a chiral molecule, known as …

Multiple optical trap** and binding: new routes to self-assembly

T Čižmár, LCD Romero, K Dholakia… - Journal of Physics B …, 2010 - iopscience.iop.org
The impact of optical forces in the physical and biological sciences now enables the
manipulation of objects ranging in size from a cell down to a single atom. The mechanical …

Chirality and angular momentum in optical radiation

MM Coles, DL Andrews - Physical Review A—Atomic, Molecular, and Optical …, 2012 - APS
This paper develops, in precise quantum electrodynamic terms, photonic attributes of the
“optical chirality density,” one of several measures long known to be conserved quantities for …

Manipulating particles with light: radiation and gradient forces

DS Bradshaw, DL Andrews - European Journal of Physics, 2017 - iopscience.iop.org
The manipulation of matter with electromagnetic radiation is a capacity that has been known
for over a century. However, the prominence of such optical effects only grew rapidly …

Hyper-Rayleigh scattering optical activity: Theory, symmetry considerations, and quantum chemistry applications

A Bonvicini, KA Forbes, DL Andrews… - The Journal of chemical …, 2023 - pubs.aip.org
This work reports on the first computational quantum-chemistry implementation of the hyper-
Rayleigh scattering optical activity (HRS-OA), a nonlinear chiroptical phenomenon. First …

Quantum formulation for nanoscale optical and material chirality: symmetry issues, space and time parity, and observables

DL Andrews - Journal of Optics, 2018 - iopscience.iop.org
To properly represent the interplay and coupling of optical and material chirality at the
photon-molecule or photon-nanoparticle level invites a recognition of quantum facets in the …

On optical vortex interactions with chiral matter

DL Andrews, LCD Romero, M Babiker - Optics Communications, 2004 - Elsevier
We examine the possibility that optical vortices should offer a controllable specificity in their
interactions with chiral matter, associated with orbital angular momentum transfer. By explicit …