Quantum control of molecular rotation

CP Koch, M Lemeshko, D Sugny - Reviews of Modern Physics, 2019 - APS
The angular momentum of molecules, or, equivalently, their rotation in three-dimensional
space, is ideally suited for quantum control. Molecular angular momentum is naturally …

[HTML][HTML] Matter manipulation with extreme terahertz light: Progress in the enabling THz technology

P Salén, M Basini, S Bonetti, J Hebling, M Krasilnikov… - Physics reports, 2019 - Elsevier
Terahertz (THz) light has proven to be a fine tool to probe and control quasi-particles and
collective excitations in solids, to drive phase transitions and associated changes in material …

Quantum coherent control of a single molecular-polariton rotation

LB Fan, CC Shu, D Dong, J He, NE Henriksen… - Physical Review Letters, 2023 - APS
We present a combined analytical and numerical study for coherent terahertz control of a
single molecular polariton, formed by strongly coupling two rotational states of a molecule …

Terahertz-induced field-free orientation of rotationally excited molecules

KN Egodapitiya, S Li, RR Jones - Physical Review Letters, 2014 - APS
We have used picosecond THz pulses to induce transient field-free orientation of OCS
molecules. Coherent optical Raman excitation prepares the molecules in rotational …

Quantum control of field-free molecular orientation

QQ Hong, ZZ Lian, CC Shu… - Physical Chemistry …, 2023 - pubs.rsc.org
Generating field-free (non-stationary) orientation of molecules in space has been a
longstanding goal in the field of quantum control of molecular rotation, which has significant …

Effect of molecular alignment and orientation on elliptically polarized high-order harmonic generation

R Zhang, F Wang, H Yuan, S Chen, C Yang, T Ou… - Physical Review A, 2024 - APS
We present a theoretical investigation of the influence of molecular alignment and
orientation on elliptically polarized high-order harmonic generation (HHG) from CO …

Rotational control of asymmetric molecules: dipole-versus polarizability-driven rotational dynamics

R Damari, S Kallush, S Fleischer - Physical review letters, 2016 - APS
We experimentally study the optical-and terahertz-induced rotational dynamics of
asymmetric molecules in the gas phase. Terahertz and optical fields are identified as two …

Orientational quantum revivals induced by a single-cycle terahertz pulse

CC Shu, QQ Hong, Y Guo, NE Henriksen - Physical Review A, 2020 - APS
The phenomenon of quantum revivals resulting from the self-interference of wave packets
has been observed in several quantum systems and utilized widely in spectroscopic …

Generation of maximal three-state field-free molecular orientation with terahertz pulses

QQ Hong, LB Fan, CC Shu, NE Henriksen - Physical Review A, 2021 - APS
We present a combined analytical and numerical investigation to show how an optimal
control field can be designed to generate maximum field-free orientation of molecules for …

Long-lasting molecular orientation induced by a single terahertz pulse

L Xu, I Tutunnikov, E Gershnabel, Y Prior… - Physical Review Letters, 2020 - APS
We present a novel, previously unreported phenomenon appearing in a thermal gas of
nonlinear polar molecules excited by a single THz pulse. We find that the induced …