Molecular main group metal hydrides

MMD Roy, AA Omana, ASS Wilson, MS Hill… - Chemical …, 2021 - ACS Publications
This review serves to document advances in the synthesis, versatile bonding, and reactivity
of molecular main group metal hydrides within Groups 1, 2, and 12–16. Particular attention …

Dihydrogen and Ethylene Activation by a Sterically Distorted Distibene

Y Pang, M Leutzsch, N Nöthling… - Angewandte Chemie …, 2023 - Wiley Online Library
Herein, we report the synthesis of a sterically distorted distibene ([4] 2) and its transition‐
metal‐like reactivity towards two fundamental feedstock chemicals: H2 and ethylene …

Hydrostibination

KM Marczenko, JA Zurakowski, KL Bamford… - Angewandte …, 2019 - Wiley Online Library
A rigid naphthalenediamine framework has been used to prepare antimony hydrides that
feature LUMO shapes and energies similar to those found in secondary boranes. By …

Isolation of 1, 2, 4, 3-triazaborol-3-yl-metal (Li, Mg, Al, Au, Zn, Sb, Bi) derivatives and reactivity toward CO and isonitriles

W Lu, H Hu, Y Li, R Ganguly… - Journal of the American …, 2016 - ACS Publications
3, 4-dihydro-2 H-1, 2, 4, 3-triazaborol-3-yl-lithium 3 was synthesized and fully characterized.
The 11B NMR spectrum, X-ray diffraction analysis, and computational studies revealed the …

Synthesis of bismuthanyl-substituted monomeric triel hydrides

R Szlosek, C Marquardt, O Hegen, G Balázs… - Chemical …, 2024 - pubs.rsc.org
The syntheses and characterizations of the first bismuthanylborane monomers stabilized
only by a donor in D· BH2Bi (SiMe3) 2 (D= DMAP 1a, IDipp 1b, IMe41c; DMAP= 4 …

Actinide–Pnictide (An− Pn) Bonds Spanning Non‐Metal, Metalloid, and Metal Combinations (An= U, Th; Pn= P, As, Sb, Bi)

TM Rookes, EP Wildman, G Balazs… - Angewandte Chemie …, 2018 - Wiley Online Library
The synthesis and characterisation is presented of the compounds [An (TrenDMBS){Pn
(SiMe3) 2}] and [An (TrenTIPS){Pn (SiMe3) 2}][TrenDMBS= N (CH2CH2NSiMe2But) 3, An …

A Mechanistic Study on Reactions of Group 13 Diyls LM with Cp*SbX2: From Stibanyl Radicals to Antimony Hydrides

C Helling, C Wölper, GE Cutsail III… - … A European Journal, 2020 - Wiley Online Library
Abstract Oxidative addition of Cp* SbX2 (X= Cl, Br, I; Cp*= C5Me5) to group 13 diyls LM (M=
Al, Ga, In; L= HC [C (Me) N (Dip)] 2, Dip= 2, 6‐iPr2C6H3) yields elemental antimony (M= Al) …

Titanium‐Catalyzed Polymerization of a Lewis Base‐Stabilized Phosphinoborane

J Braese, F Lehnfeld, VT Annibale… - … A European Journal, 2023 - Wiley Online Library
The reaction of the Lewis base‐stabilized phosphinoborane monomer tBuHPBH2NMe3 (2
a) with catalytic amounts of bis (η5: η1‐adamantylidenepentafulvene) titanium (1) provides a …

Synthesis and Application of Alkali Metal Antimonide—A New Approach to Antimony Chemistry

K Dollberg, S Schneider, RM Richter… - Angewandte Chemie …, 2022 - Wiley Online Library
Alkali metal dihydrogen‐antimonides [M (L) xSbH2], short: alkali metal antimonides (M= Li,
Na, K, Rb, Cs; 1: L= pmdta; 2: L= crown‐ether), were prepared from stibine and n …

Structures and Stability of Mixed Main Group Hydrides [PBEH6]n (E = C, Si, Ge; n = 1–4) and Donor–Acceptor Stabilization of Monomeric Chain Isomers

AM Belousova, AY Timoshkin - The Journal of Physical Chemistry …, 2023 - ACS Publications
Structures and stability of mixed group 13–14–15 element hydrides PBEH6 (E= C, Si, Ge),
their oligomers, and complexes with Lewis acids and Lewis base are computationally …