Laser ablation plasmas and spectroscopy for nuclear applications

EH Kwapis, J Borrero, KS Latty, HB Andrews… - Applied …, 2024 - opg.optica.org
The development of measurement methodologies to detect and monitor nuclear-relevant
materials remains a consistent and significant interest across the nuclear energy …

Applications of laser-induced breakdown spectroscopy in industrial measurement and monitoring: Multi-technology combination

M Cui, S **ong, N Yang, Y Wang, Z Wang… - Applied Spectroscopy …, 2024 - Taylor & Francis
As a crucial detection technology in the era of digital transformation, laser induced
breakdown spectroscopy (LIBS) has been widely used in industrial measurement and …

[HTML][HTML] Optical spectroscopy of laser-produced plasmas for standoff isotopic analysis

SS Harilal, BE Brumfield, NL LaHaye… - Applied Physics …, 2018 - pubs.aip.org
Rapid, in-field, and non-contact isotopic analysis of solid materials is extremely important to
a large number of applications, such as nuclear nonproliferation monitoring and forensics …

Physical conditions for UO formation in laser-produced uranium plumes

SS Harilal, EJ Kautz, BE Bernacki… - Physical Chemistry …, 2019 - pubs.rsc.org
We investigate the oxidation of uranium (U) species, the physical conditions leading to
uranium monoxide (UO) formation and the interplay between plume hydrodynamics and …

Hyperfine structures and isotopic shifts of uranium transitions using tunable laser spectroscopy of laser ablation plumes

SS Harilal, CM Murzyn, MC Phillips… - Spectrochimica Acta Part B …, 2020 - Elsevier
We report isotopic shifts and hyperfine structures of selected U transitions employing tunable
spectroscopy viz: laser-induced fluorescence and laser absorption spectroscopy of laser …

Early-and late-time dynamics of laser-produced plasmas by combining emission and absorption spectroscopy

NL LaHaye, SS Harilal, MC Phillips - Spectrochimica Acta Part B: Atomic …, 2021 - Elsevier
Optical emission spectroscopy and laser absorption spectroscopy are two highly
complementary techniques for diagnosing plasmas, specifically determining important …

Experimental and computational investigation into the hydrodynamics and chemical dynamics of laser ablation aluminum plasmas

EH Kwapis, JW Posey, E Medici, K Berg… - Physical Chemistry …, 2023 - pubs.rsc.org
Laser ablation plasma chemistry is governed by a complex interplay between hydrodynamic
plasma-gas mixing processes, thermodynamics, and rapid high-temperature chemical …

[HTML][HTML] Laser-induced fluorescence of filament-produced plasmas

EJ Kautz, MC Phillips, SS Harilal - Journal of Applied Physics, 2021 - pubs.aip.org
Self-guided ultrafast laser filaments are a promising method for laser beam delivery and
plasma generation for standoff and remote detection of elements and isotopes via filament …

Shock physics and shadowgraphic measurements of laser-produced cerium plasmas

EH Kwapis, M Hewitt, KC Hartig - Optics Express, 2023 - opg.optica.org
Shadowgraphic measurements are combined with theory on gas-dynamics to investigate
the shock physics associated with nanosecond laser ablation of cerium metal targets. Time …

Elucidating uranium monoxide spectral features from a laser-produced plasma

SS Harilal, BE Brumfield, N Glumac, MC Phillips - Optics express, 2018 - opg.optica.org
Uranium, because of its pyrophoricity, oxidizes rapidly in an oxygen-containing high-
temperature environment. However, so far, the identification of uranium oxide (UO) emission …