Confinement of luminescent guests in metal–organic frameworks: understanding pathways from synthesis and multimodal characterization to potential applications of …

M Gutiérrez, Y Zhang, JC Tan - Chemical Reviews, 2022 - ACS Publications
This review gives an authoritative, critical, and accessible overview of an emergent class of
fluorescent materials termed “LG@ MOF”, engineered from the nanoscale confinement of …

Origin of ferroelectricity in two prototypical hybrid organic–inorganic perovskites

K Li, ZG Li, J Xu, Y Qin, W Li, A Stroppa… - Journal of the …, 2022 - ACS Publications
Hybrid organic–inorganic perovskite (HOIP) ferroelectrics are attracting considerable
interest because of their high performance, ease of synthesis, and lightweight. However, the …

Rational Design of 2D Metal Halide Perovskites with Low Congruent Melting Temperature and Large Melt-Processable Window

W Wang, CD Liu, CC Fan, XB Fu, CQ **g… - Journal of the …, 2024 - ACS Publications
Metal halide perovskites (MHPs) have garnered significant attention due to their distinctive
optical and electronic properties, coupled with excellent processability. However, the …

Entropy-driven stabilization of the cubic phase of MaPbI 3 at room temperature

A Bonadio, CA Escanhoela, FP Sabino… - Journal of Materials …, 2021 - pubs.rsc.org
Methylammonium lead iodide (MAPbI3) is an important light-harvesting semiconducting
material for solar-cell devices. We investigate the effect of long thermal annealing in an inert …

Free energy predictions for crystal stability and synthesisability

K Tolborg, J Klarbring, AM Ganose, A Walsh - Digital Discovery, 2022 - pubs.rsc.org
What is the likelihood that a hypothetical material—the combination of a composition and
crystal structure—can be formed? Underpinning the reliability of predictions for local or …

Exploring Librational Pathways with on-the-Fly Machine-Learning Force Fields: Methylammonium Molecules in MAPbX3 (X = I, Br, Cl) Perovskites

M Bokdam, J Lahnsteiner… - The Journal of Physical …, 2021 - ACS Publications
Two seemingly similar crystal structures of the low-temperature (∼ 100 K) MAPbX3 (X= I, Br,
Cl) perovskites, but with different relative methylammonium (MA) ordering, have appeared …

Metal-free perovskites for non linear optical materials

TW Kasel, Z Deng, AM Mroz, CH Hendon, KT Butler… - Chemical …, 2019 - pubs.rsc.org
We identify the existence of non linear optical (NLO) activity in a number of novel ABX3-type
metal-free perovskites, where A is a highly tuneable organic cation, B is a NH4 cation and X …

Pressure-induced non-radiative losses in halide perovskite light-emitting diodes

YK Jung, M Abdulla, RH Friend, SD Stranks… - Journal of Materials …, 2022 - pubs.rsc.org
The control of non-radiative losses in light-emitting diodes (LEDs) based on metal halide
perovskites is crucial to improve device efficiency. Recent studies have shown a correlation …

Experimental evidence for vibrational entropy as driving parameter of flexibility in the metal–organic framework ZIF-4 (Zn)

KT Butler, P Vervoorts, MG Ehrenreich… - Chemistry of …, 2019 - ACS Publications
Large structural flexibility in some metal–organic frameworks (MOFs) is not only fascinating
from a fundamental point of view but offers exciting opportunities in the areas of gas sensing …

The Advantages of Flexibility: The Role of Entropy in Crystal Structures Containing C–H··· F Interactions

CJG Wilson, J Plesniar, H Kuhn… - Crystal Growth & …, 2024 - ACS Publications
Molecular crystal structures are often interpreted in terms of strong, structure directing,
intermolecular interactions, especially those with distinct geometric signatures such as H …