Relativistic orbital-optimized density functional theory for accurate core-level spectroscopy

LA Cunha, D Hait, R Kang, Y Mao… - The Journal of …, 2022 - ACS Publications
Core-level spectra of 1s electrons of elements heavier than Ne show significant relativistic
effects. We combine advances in orbital-optimized density functional theory (OO-DFT) with …

Accurate core excitation and ionization energies from a state-specific coupled-cluster singles and doubles approach

JE Arias-Martinez, LA Cunha, KJ Oosterbaan… - Physical Chemistry …, 2022 - pubs.rsc.org
We investigate the use of orbital-optimized references in conjunction with single-reference
coupled-cluster theory with single and double substitutions (CCSD) for the study of core …

Reference Energies for Valence Ionizations and Satellite Transitions

A Marie, PF Loos - Journal of Chemical Theory and Computation, 2024 - ACS Publications
Upon ionization of an atom or a molecule, another electron (or more) can be simultaneously
excited. These concurrently generated states are called “satellites”(or shakeup transitions) …

X-ray induced electron and ion fragmentation dynamics in IBr

PJ Ho, D Ray, CS Lehmann, AEA Fouda… - The Journal of …, 2023 - pubs.aip.org
Characterization of the inner-shell decay processes in molecules containing heavy elements
is key to understanding x-ray damage of molecules and materials and for medical …

MP2-based composite extrapolation schemes can predict core-ionization energies for first-row elements with coupled-cluster level accuracy

A Morgunov, HK Tran, OR Meitei… - The Journal of …, 2024 - ACS Publications
X-ray photoelectron spectroscopy (XPS) measures core–electron binding energies (CEBEs)
to reveal element-specific insights into the chemical environment and bonding. Accurate …

Efficient Spin-Adapted Implementation of Multireference Algebraic Diagrammatic Construction Theory. I. Core-Ionized States and X-ray Photoelectron Spectra

CEV de Moura, AY Sokolov - The Journal of Physical Chemistry A, 2024 - ACS Publications
We present an efficient implementation of multireference algebraic diagrammatic
construction theory (MR-ADC) for simulating core-ionized states and X-ray photoelectron …

Real-Space Pseudopotential Method for the Calculation of Third-Row Elements X-ray Photoelectron Spectroscopic Signatures

L Liu, Q Xu, L dos Anjos Cunha, H **n… - Journal of Chemical …, 2024 - ACS Publications
X-ray photoelectron spectroscopy (XPS) is a powerful characterization technique that
unveils subtle chemical environment differences via core–electron binding energy (CEBE) …

Elucidating Anomalous Intensity Ratios in Chlorine L-Edge X-ray Absorption Spectroscopy: Multiplet Effects and Core Rydberg Transitions

Z Lin, J Liu, C Zhang, X Zheng… - The Journal of Physical …, 2024 - ACS Publications
A relativistic core–valence-separated equation-of-motion coupled cluster (CVS-EOM-CC)
study of chlorine L2, 3-edge X-ray absorption near-edge structure (XANES) spectra using …

Estimating vertical core-excitation energies from Møller–Plesset theory with spin projection

AY Zamani, HP Hratchian - Molecular Physics, 2024 - Taylor & Francis
Spin projected ΔUHF and ΔUMP n (n= 2, 2.5, 3) methods are used to calculate vertical core
excitation energies. These methods are applied to a set of symmetrical molecules with …

DEVELOPMENT OF RELATIVISTIC COUPLED-CLUSTER TECHNIQUES FOR X-RAY SPECTROSCOPY

X Zheng - 2023 - jscholarship.library.jhu.edu
The dissertation is focused on development of relativistic coupled-cluster (CC) techniques
aiming to accurately calculate x-ray photoelectron and absorption spectroscopy. The …