The acidity of atmospheric particles and clouds

HOT Pye, A Nenes, B Alexander, AP Ault… - Atmospheric …, 2020 - acp.copernicus.org
Acidity, defined as pH, is a central component of aqueous chemistry. In the atmosphere, the
acidity of condensed phases (aerosol particles, cloud water, and fog droplets) governs the …

Recent advances in understanding secondary organic aerosol: Implications for global climate forcing

M Shrivastava, CD Cappa, J Fan… - Reviews of …, 2017 - Wiley Online Library
Anthropogenic emissions and land use changes have modified atmospheric aerosol
concentrations and size distributions over time. Understanding preindustrial conditions and …

Reactive nitrogen chemistry in aerosol water as a source of sulfate during haze events in China

Y Cheng, G Zheng, C Wei, Q Mu, B Zheng, Z Wang… - Science …, 2016 - science.org
Fine-particle pollution associated with winter haze threatens the health of more than 400
million people in the North China Plain. Sulfate is a major component of fine haze particles …

Highly acidic ambient particles, soluble metals, and oxidative potential: a link between sulfate and aerosol toxicity

T Fang, H Guo, L Zeng, V Verma… - … science & technology, 2017 - ACS Publications
Soluble transition metals in particulate matter (PM) can generate reactive oxygen species in
vivo by redox cycling, leading to oxidative stress and adverse health effects. Most metals …

Rapid transition in winter aerosol composition in Bei**g from 2014 to 2017: response to clean air actions

H Li, J Cheng, Q Zhang, B Zheng… - Atmospheric …, 2019 - acp.copernicus.org
The clean air actions implemented by the Chinese government in 2013 have led to
significantly improved air quality in Bei**g. In this work, we combined the in situ …

Fine-particle pH for Bei**g winter haze as inferred from different thermodynamic equilibrium models

S Song, M Gao, W Xu, J Shao, G Shi… - Atmospheric …, 2018 - acp.copernicus.org
pH is an important property of aerosol particles but is difficult to measure directly. Several
studies have estimated the pH values for fine particles in northern China winter haze using …

Aerosol pH and its driving factors in Bei**g

J Ding, P Zhao, J Su, Q Dong, X Du… - … Chemistry and Physics, 2019 - acp.copernicus.org
Aerosol acidity plays a key role in secondary aerosol formation. The high-temporal-
resolution PM 2.5 pH and size-resolved aerosol pH in Bei**g were calculated with …

High aerosol acidity despite declining atmospheric sulfate concentrations over the past 15 years

RJ Weber, H Guo, AG Russell, A Nenes - Nature Geoscience, 2016 - nature.com
Particle acidity affects aerosol concentrations, chemical composition and toxicity. Sulfate is
often the main acid component of aerosols, and largely determines the acidity of fine …

[HTML][HTML] Formation mechanisms of atmospheric nitrate and sulfate during the winter haze pollution periods in Bei**g: gas-phase, heterogeneous and aqueous-phase …

P Liu, C Ye, C Xue, C Zhang, Y Mu… - … Chemistry and Physics, 2020 - acp.copernicus.org
A vast area in China is currently going through severe haze episodes with drastically
elevated concentrations of PM 2.5 in winter. Nitrate and sulfate are the main constituents of …

Revising the hygroscopicity of inorganic sea salt particles

P Zieger, O Väisänen, JC Corbin, DG Partridge… - Nature …, 2017 - nature.com
Sea spray is one of the largest natural aerosol sources and plays an important role in the
Earth's radiative budget. These particles are inherently hygroscopic, that is, they take-up …