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Molecular photodissociation dynamics revealed by Coulomb explosion imaging
Coulomb explosion imaging (CEI) methods are finding ever-growing use as a means of
exploring and distinguishing the static stereo-configurations of small quantum systems …
exploring and distinguishing the static stereo-configurations of small quantum systems …
[HTML][HTML] Perspective: Fundamental aspects of time-dependent density functional theory
In the thirty-two years since the birth of the foundational theorems, time-dependent density
functional theory has had a tremendous impact on calculations of electronic spectra and …
functional theory has had a tremendous impact on calculations of electronic spectra and …
Two-electron Rabi oscillations in real-time time-dependent density-functional theory
We investigate the Rabi oscillations of electrons excited by an applied electric field in
several simple molecular systems using time-dependent configuration interaction (TDCI) …
several simple molecular systems using time-dependent configuration interaction (TDCI) …
Multiparticle cumulant map** for Coulomb explosion imaging
We extend covariance velocity map ion imaging to four particles, establishing cumulant
map** and allowing for measurements that provide insights usually associated with …
map** and allowing for measurements that provide insights usually associated with …
Tabletop imaging of structural evolutions in chemical reactions demonstrated for the acetylene cation
The introduction of femto-chemistry has made it a primary goal to follow the nuclear and
electronic evolution of a molecule in time and space as it undergoes a chemical reaction …
electronic evolution of a molecule in time and space as it undergoes a chemical reaction …
X-ray induced Coulomb explosion imaging of transient excited-state structural rearrangements in CS2
Structural imaging of transient excited-state species is a key goal of molecular physics,
promising to unveil rich information about the dynamics underpinning photochemical …
promising to unveil rich information about the dynamics underpinning photochemical …
Native frames: Disentangling sequential from concerted three-body fragmentation
A key question concerning the three-body fragmentation of polyatomic molecules is the
distinction of sequential and concerted mechanisms, ie, the stepwise or simultaneous …
distinction of sequential and concerted mechanisms, ie, the stepwise or simultaneous …
Filming enhanced ionization in an ultrafast triatomic slingshot
Filming atomic motion within molecules is an active pursuit of molecular physics and
quantum chemistry. A promising method is laser-induced Coulomb Explosion Imaging (CEI) …
quantum chemistry. A promising method is laser-induced Coulomb Explosion Imaging (CEI) …
Nonsequential and Sequential Fragmentation of in Intense Laser Fields
We experimentally studied the three-body fragmentation dynamics of CO 2 initiated by
intense femtosecond laser pulses. Sequential and nonsequential fragmentations were …
intense femtosecond laser pulses. Sequential and nonsequential fragmentations were …
[HTML][HTML] Exact factorization adventures: A promising approach for non-bound states
Modeling the dynamics of non-bound states in molecules requires an accurate description of
how electronic motion affects nuclear motion and vice-versa. The exact factorization (XF) …
how electronic motion affects nuclear motion and vice-versa. The exact factorization (XF) …