Quantum control of molecular rotation

CP Koch, M Lemeshko, D Sugny - Reviews of Modern Physics, 2019 - APS
The angular momentum of molecules, or, equivalently, their rotation in three-dimensional
space, is ideally suited for quantum control. Molecular angular momentum is naturally …

Manipulation of molecules with electromagnetic fields

M Lemeshko, RV Krems, JM Doyle, S Kais - Molecular Physics, 2013 - Taylor & Francis
The goal of the present article is to review the major developments that have led to the
current understanding of molecule–field interactions and experimental methods for …

Following a chemical reaction using high-harmonic interferometry

HJ Wörner, JB Bertrand, DV Kartashov, PB Corkum… - Nature, 2010 - nature.com
The study of chemical reactions on the molecular (femtosecond) timescale typically uses
pump laser pulses to excite molecules and subsequent probe pulses to interrogate them …

Photoelectron angular distributions from strong-field ionization of oriented molecules

L Holmegaard, JL Hansen, L Kalhøj, S Louise Kragh… - Nature Physics, 2010 - nature.com
The combination of ultrafast light sources with detection of molecular-frame photoelectron
angular distributions (MFPADs) is setting new standards for detailed interrogation of …

Strong-field rescattering physics—self-imaging of a molecule by its own electrons

CD Lin, AT Le, Z Chen, T Morishita… - Journal of Physics B …, 2010 - iopscience.iop.org
When an atom or molecule is exposed to a short intense laser pulse, electrons that were
removed at an earlier time may be driven back by the oscillating electric field of the laser to …

Diffractive imaging of coherent nuclear motion in isolated molecules

J Yang, M Guehr, X Shen, R Li, T Vecchione, R Coffee… - Physical review …, 2016 - APS
Observing the motion of the nuclear wave packets during a molecular reaction, in both
space and time, is crucial for understanding and controlling the outcome of photoinduced …

Tracing orbital images on ultrafast time scales

R Wallauer, M Raths, K Stallberg, L Münster… - Science, 2021 - science.org
Frontier orbitals determine fundamental molecular properties such as chemical reactivities.
Although electron distributions of occupied orbitals can be imaged in momentum space by …

Capturing chemistry in action with electrons: realization of atomically resolved reaction dynamics

AA Ischenko, PM Weber, RJD Miller - Chemical reviews, 2017 - ACS Publications
One of the grand challenges in chemistry has been to directly observe atomic motions
during chemical processes. The depiction of the nuclear configurations in space-time to …

Conical Intersection Dynamics in NO2 Probed by Homodyne High-Harmonic Spectroscopy

HJ Wörner, JB Bertrand, B Fabre, J Higuet, H Ruf… - Science, 2011 - science.org
Conical intersections play a crucial role in the chemistry of most polyatomic molecules,
ranging from the simplest bimolecular reactions to the photostability of DNA. The real-time …

Time-resolved imaging of purely valence-electron dynamics during a chemical reaction

P Hockett, CZ Bisgaard, OJ Clarkin, A Stolow - Nature Physics, 2011 - nature.com
Chemical reactions are manifestations of the dynamics of molecular valence electrons and
their couplings to atomic motions. Emerging methods in attosecond science can probe …