Coherent two-dimensional and broadband electronic spectroscopies

S Biswas, JW Kim, X Zhang, GD Scholes - Chemical Reviews, 2022 - ACS Publications
Over the past few decades, coherent broadband spectroscopy has been widely used to
improve our understanding of ultrafast processes (eg, photoinduced electron transfer, proton …

Photosynthetic light harvesting: excitons and coherence

F Fassioli, R Dinshaw, PC Arpin… - Journal of The Royal …, 2014 - royalsocietypublishing.org
Photosynthesis begins with light harvesting, where specialized pigment–protein complexes
transform sunlight into electronic excitations delivered to reaction centres to initiate charge …

Charge photogeneration in neat conjugated polymers

OG Reid, RD Pensack, Y Song, GD Scholes… - Chemistry of …, 2014 - ACS Publications
The origin and yield of charges in neat conjugated polymers has long been controversial. In
this paper, we review the body of literature that has been created over the past three …

Methylene blue exciton states steer nonradiative relaxation: Ultrafast spectroscopy of methylene blue dimer

JC Dean, DG Oblinsky, SR Rather… - The Journal of Physical …, 2016 - ACS Publications
The photochemistry and aggregation properties of methylene blue (MB) lead to its popular
use in photodynamic therapy. The facile formation of strongly coupled “face-to-face” H …

Coherence spectroscopy in the condensed phase: Insights into molecular structure, environment, and interactions

JC Dean, GD Scholes - Accounts of chemical research, 2017 - ACS Publications
Conspectus The role of coherences, or coherently excited superposition states, in complex
condensed-phase systems has been the topic of intense interest and debate for a number of …

The separation of vibrational coherence from ground-and excited-electronic states in P3HT film

Y Song, C Hellmann, N Stingelin… - The Journal of chemical …, 2015 - pubs.aip.org
Concurrence of the vibrational coherence and ultrafast electron transfer has been observed
in polymer/fullerene blends. However, it is difficult to experimentally investigate the role that …

Extracting the frequency-dependent dynamic stokes shift from two-dimensional electronic spectra with prominent vibrational coherences

J Lu, Y Lee, JM Anna - The Journal of Physical Chemistry B, 2020 - ACS Publications
The dynamic Stokes shift is a common means for characterizing ultrafast solvation dynamics
of electronically excited states. Here we extract the excitation frequency-dependent dynamic …

Broadband transient absorption and two-dimensional electronic spectroscopy of methylene blue

JC Dean, SR Rather, DG Oblinsky… - The Journal of …, 2015 - ACS Publications
Broadband transient absorption and two-dimensional electronic spectroscopy (2DES)
studies of methylene blue in aqueous solution are reported. By isolating the coherent …

Ultrafast solvation dynamics and vibrational coherences of halogenated boron-dipyrromethene derivatives revealed through two-dimensional electronic spectroscopy

Y Lee, S Das, RM Malamakal, S Meloni… - Journal of the …, 2017 - ACS Publications
Boron-dipyrromethene (BODIPY) chromophores have a wide range of applications,
spanning areas from biological imaging to solar energy conversion. Understanding the …

Efficient charge generation via hole transfer in dilute organic donor–fullerene blends

Y Song, A Schubert, X Liu, S Bhandari… - The Journal of …, 2020 - ACS Publications
Efficient organic photovoltaics (OPVs) require broadband charge photogeneration with near-
unity quantum yield. This can only be achieved by exploiting all pathways that generate …