Manganese-catalyzed hydrogenation, dehydrogenation, and hydroelementation reactions

K Das, S Waiba, A Jana, B Maji - Chemical Society Reviews, 2022‏ - pubs.rsc.org
The emerging field of organometallic catalysis has shifted towards research on Earth-
abundant transition metals due to their ready availability, economic advantage, and novel …

Borrowing hydrogen for organic synthesis

BG Reed-Berendt, DE Latham, MB Dambatta… - ACS central …, 2021‏ - ACS Publications
Borrowing hydrogen is a process that is used to diversify the synthetic utility of commodity
alcohols. A catalyst first oxidizes an alcohol by removing hydrogen to form a reactive …

Alcohols as substrates in transition-metal-catalyzed arylation, alkylation, and related reactions

A Cook, SG Newman - Chemical Reviews, 2024‏ - ACS Publications
Alcohols are abundant and attractive feedstock molecules for organic synthesis. Many
methods for their functionalization require them to first be converted into a more activated …

3d-Metal catalyzed N-and C-alkylation reactions via borrowing hydrogen or hydrogen autotransfer

T Irrgang, R Kempe - Chemical reviews, 2018‏ - ACS Publications
The conservation of our element resources is a fundamental challenge of mankind. The
development of alcohol refunctionalization reactions is a possible fossil carbon conservation …

Homogeneous manganese-catalyzed hydrogenation and dehydrogenation reactions

Y Wang, M Wang, Y Li, Q Liu - Chem, 2021‏ - cell.com
The development of novel and efficient earth-abundant metal catalysts as inexpensive and
sustainable alternatives to noble-metal catalysts is a rapidly expanding and evolving field of …

Enable biomass-derived alcohols mediated alkylation and transfer hydrogenation

X Liu, L Huang, Y Ma, G She, P Zhou, L Zhu… - Nature …, 2024‏ - nature.com
A single-atom catalyst with generally regarded inert Zn–N4 motifs derived from ZIF-8 is
unexpectedly efficient for the activation of alcohols, enabling alcohol-mediated alkylation …

Towards ligand simplification in manganese-catalyzed hydrogenation and hydrosilylation processes

ES Gulyaeva, ES Osipova, R Buhaibeh… - Coordination Chemistry …, 2022‏ - Elsevier
Rapidly emerging application of organometallic manganese complexes incorporating less
elaborated mono-and bidentate donor ligands in catalytic hydrogenation, transfer …

Sustainable synthesis of quinazoline and 2-aminoquinoline via dehydrogenative coupling of 2-aminobenzyl alcohol and nitrile catalyzed by phosphine-free …

K Das, A Mondal, D Pal, D Srimani - Organic Letters, 2019‏ - ACS Publications
A sustainable synthesis of quinazoline and 2-aminoquinoline via acceptorless
dehydrogenative annulation is presented. The reaction is catalyzed by earth-abundant well …

Recent advancement in oxidation or acceptorless dehydrogenation of alcohols to valorised products using manganese based catalysts

P Chandra, T Ghosh, N Choudhary… - Coordination Chemistry …, 2020‏ - Elsevier
Manganese based compounds have gained much interest as catalytic materials due to their
natural abundance, biocompatibility, and multiple oxidation states. Manganese-based …

Catalytic C1 Alkylation with Methanol and Isotope‐Labeled Methanol

J Sklyaruk, JC Borghs, O El‐Sepelgy… - Angewandte …, 2019‏ - Wiley Online Library
A metal‐catalyzed methylation process has been developed. By employing an air‐and
moisture‐stable manganese catalyst together with isotopically labeled methanol, a series of …