Computational design of magnetic molecules and their environment using quantum chemistry, machine learning and multiscale simulations

A Lunghi, S Sanvito - Nature Reviews Chemistry, 2022‏ - nature.com
Having served as a playground for fundamental studies on the physics of d and f electrons
for almost a century, magnetic molecules are now becoming increasingly important for …

The OpenMolcas Web: A Community-Driven Approach to Advancing Computational Chemistry

G Li Manni, I Fdez. Galván, A Alavi… - Journal of chemical …, 2023‏ - ACS Publications
The developments of the open-source OpenMolcas chemistry software environment since
spring 2020 are described, with a focus on novel functionalities accessible in the stable …

Open-source machine learning in computational chemistry

A Hagg, KN Kirschner - Journal of chemical information and …, 2023‏ - ACS Publications
The field of computational chemistry has seen a significant increase in the integration of
machine learning concepts and algorithms. In this Perspective, we surveyed 179 open …

Block2: A comprehensive open source framework to develop and apply state-of-the-art DMRG algorithms in electronic structure and beyond

H Zhai, HR Larsson, S Lee, ZH Cui, T Zhu… - The Journal of …, 2023‏ - pubs.aip.org
block2 is an open source framework to implement and perform density matrix
renormalization group and matrix product state algorithms. Out-of-the-box it supports the …

A perspective on sustainable computational chemistry software development and integration

R Di Felice, ML Mayes, RM Richard… - Journal of chemical …, 2023‏ - ACS Publications
The power of quantum chemistry to predict the ground and excited state properties of
complex chemical systems has driven the development of computational quantum chemistry …

Influence of pump laser fluence on ultrafast myoglobin structural dynamics

TRM Barends, A Gorel, S Bhattacharyya, G Schirò… - Nature, 2024‏ - nature.com
High-intensity femtosecond pulses from an X-ray free-electron laser enable pump–probe
experiments for the investigation of electronic and nuclear changes during light-induced …

How will quantum computers provide an industrially relevant computational advantage in quantum chemistry?

VE Elfving, BW Broer, M Webber, J Gavartin… - arxiv preprint arxiv …, 2020‏ - arxiv.org
Numerous reports claim that quantum advantage, which should emerge as a direct
consequence of the advent of quantum computers, will herald a new era of chemical …

Molecular Network Approach to Anisotropic Ising Lattices: Parsing Magnetization Dynamics in Er3+ Systems with 0–3-Dimensional Spin Interactivity

AP Orlova, MS Varley, MG Bernbeck… - Journal of the …, 2023‏ - ACS Publications
We present a wide-ranging interrogation of the border between single-molecule and solid-
state magnetism through a study of erbium-based Ising-type magnetic compounds with a …

Slow magnetic relaxation in a europium (II) complex

D Errulat, KLM Harriman, DA Gálico… - Nature …, 2024‏ - nature.com
Single-ion anisotropy is vital for the observation of Single-Molecule Magnet (SMM)
properties (ie, a slow dynamics of the magnetization) in lanthanide-based systems. In the …

Designing quantum spaces of higher dimensionality from a tetranuclear erbium-based single-molecule magnet

AP Orlova, MG Bernbeck… - Journal of the American …, 2024‏ - ACS Publications
The spin relaxation of an Er3+ tetranuclear single-molecule magnet,[Er (hdcCOT) I]
4,(hdcCOT= hexahydrodicyclopentacyclooctatetraenide dianion), is modeled as a near …