Catalyst stability considerations for electrochemical energy conversion with non-noble metals: do we measure on what we synthesized?

D Hochfilzer, I Chorkendorff, J Kibsgaard - ACS Energy Letters, 2023 - ACS Publications
Working with non-noble electrocatalysts poses significant experimental challenges to
unambiguously evaluate their intrinsic activity and characterize their working state and …

Morphological stability of copper surfaces under reducing conditions

SJ Raaijman, N Arulmozhi… - ACS Applied Materials & …, 2021 - ACS Publications
Though copper is a capable electrocatalyst for the CO2 reduction reaction (CO2RR), it
rapidly deactivates to produce mostly hydrogen. A current hypothesis as to why this occurs is …

Dynamic Ionization Equilibrium-Induced “Oxygen Exchange” in CO Electroreduction

H Zhang, Y Cui, C Ren, Q Li, C Ling, J Wang - ACS Catalysis, 2024 - ACS Publications
The oxygen source of oxygenates is the fundamental issue for CO2/CO electroreduction,
which was firmly believed to originate from the gas feed (Ogas) for a long time. However …

Ab initio-based modeling of thermodynamic cyclic voltammograms: a benchmark study on Ag (100) in bromide solutions

N Bergmann, NG Hörmann… - Journal of Chemical …, 2023 - ACS Publications
Experimental cyclic voltammograms (CVs) measured in the slow scan rate limit can be
entirely described in terms of the thermodynamic equilibrium quantities of the electrified …

In Situ Analysis of the Facets of Cu-Based Electrocatalysts in Alkaline Media Using Pb Underpotential Deposition

D Hochfilzer, A Tiwari, EL Clark, AS Bjørnlund… - Langmuir, 2022 - ACS Publications
Establishing relationships between the surface atomic structure and activity of Cu-based
electrocatalysts for CO2 and CO reduction is hindered by probable surface restructuring …

Effects of adsorbed OH on Pt (100)/water interfacial structures and potential

JX Zhu, JB Le, MTM Koper… - The Journal of …, 2021 - ACS Publications
Adsorbates at the electrode change the structure of the electrode/electrolyte interface.
Despite the important influence of the interfacial structure on electrochemical processes …

Clean and reproducible voltammetry of copper single crystals with prominent facet-specific features using induction annealing

SJ Raaijman, N Arulmozhi, AHM da Silva… - Journal of The …, 2021 - iopscience.iop.org
Although copper is widely used as an electrocatalyst for the CO 2 reduction reaction, often
little emphasis is placed on identifying exactly the facet distribution of the copper surface …

Insight into selectivity differences of glycerol electro-oxidation on Pt (111) and Ag (111)

Z Meng, D Tran, J Hjelm, HH Kristoffersen… - ACS …, 2024 - ACS Publications
Electro-oxidation is a way to utilize glycerol, a byproduct of biodiesel production, to produce
fuels and feedstock chemicals for the chemical industry. A significant challenge is to get …

Ab initio molecular dynamics investigation of the Pt (111)–water interface structure in an alkaline environment with high surface OH-coverages

L Partanen, K Laasonen - Physical Chemistry Chemical Physics, 2024 - pubs.rsc.org
In this study, we investigate the structure of the Pt (111)–water interface in an alkaline
environment with large OH coverages of 1/3, 2/3 and 1 monolayer using a large well …

Electrooxidation of CO on Platinum Nanoparticles Supported on NiO Thin Films

A Galyamova, H Ha, G Henkelman… - The Journal of Physical …, 2023 - ACS Publications
In this article, we report on a robust experimental model to investigate strong metal–support
interactions (SMSI) and their effect on electrocatalytic reactions in the absence and …