The role of high‐entropy materials in lithium‐based rechargeable batteries

R Guo, Y Yang, C Zhao, F Huo, J Xue… - Advanced Functional …, 2024 - Wiley Online Library
The low energy density, safety concerns, and high cost associated with conventional lithium‐
ion batteries pose challenges in meeting the growing demands of emerging applications …

Electrochemical imaging of interfaces in energy storage via scanning probe methods: techniques, applications, and prospects

A Mishra, D Sarbapalli, O Rodríguez… - Annual Review of …, 2023 - annualreviews.org
Develo** a deeper understanding of dynamic chemical, electronic, and morphological
changes at interfaces is key to solving practical issues in electrochemical energy storage …

Voltammetric detection of singlet oxygen enabled by nanogap scanning electrochemical microscopy

A Mishra, M Zorigt, DO Kim… - Journal of the American …, 2024 - ACS Publications
Despite the significance of singlet oxygen (1O2) in several biological, chemical, and energy
storage systems, its voltammetric reduction at an electrode remains unreported. We address …

Multiscale Investigation of Sodium‐Ion Battery Anodes: Analytical Techniques and Applications

D Schäfer, K Hankins, M Allion… - Advanced Energy …, 2024 - Wiley Online Library
The anode/electrolyte interface behavior, and by extension, the overall cell performance of
sodium‐ion batteries is determined by a complex interaction of processes that occur at all …

Basics of the scanning electrochemical microscope and its application in the characterization of lithium-ion batteries: a brief review

R He, L Zhou, R Tenent, M Zhou - Materials Chemistry Frontiers, 2023 - pubs.rsc.org
A scanning electrochemical microscope (SECM) can directly monitor electrochemical
processes at interfaces of electrodes and electrolytes and has been used as an analytical …

In situ Observation of Evolving H2 and Solid Electrolyte Interphase Development at Potassium Insertion Materials within Highly Concentrated Aqueous Electrolytes

ZT Gossage, N Ito, T Hosaka, R Tatara… - Angewandte …, 2023 - Wiley Online Library
The solid‐electrolyte interphase (SEI) is key to stable, high voltage lithium‐ion batteries
(LIBs) as a protective barrier that prevents electrolyte decomposition. The SEI is thought to …

Current trends in SECM for energy storage devices: reaching the microstructure level to tune devices and performance

AR Raju, SB Schougaard, J Mauzeroll - Current Opinion in …, 2024 - Elsevier
Increasing demand for sustainable energy resources necessitates the advancements of
electrochemical energy storage and conversion (EESC) devices. For optimal device …

A surface modification strategy towards reversible Na-ion intercalation on graphitic carbon using fluorinated few-layer graphene

D Sarbapalli, YH Lin, S Stafford, J Son… - Journal of The …, 2022 - iopscience.iop.org
Na-ion batteries (NIBs) are proposed as a promising candidate for beyond Li-ion
chemistries, however, a key challenge associated with NIBs is the inability to achieve …

Scanning electrochemical microscopy for chemical imaging and understanding redox activities of battery materials

LE Strange, X Li, E Wornyo… - … & Biomedical Imaging, 2023 - ACS Publications
Improving the charge storage capacity and lifetime and charging/discharging efficiency of
battery systems is essential for large-scale applications such as long-term grid storage and …

Quantifying Interfacial Ion Transfer at Operating Potassium-Insertion Battery Electrodes within Highly Concentrated Aqueous Solutions

ZT Gossage, R Tatara, T Hosaka… - ACS Applied Materials & …, 2024 - ACS Publications
Electrode/electrolyte interfacial ion transfer is a fundamental process occurring during
insertion-type redox reactions at battery electrodes. The rate at which ions move into and out …