Design of local atomic environments in single‐atom electrocatalysts for renewable energy conversionsFree GPT-4

T Sun, S Mitchell, J Li, P Lyu, X Wu… - Advanced …, 2021 - Wiley Online Library
Single‐atom electrocatalysts (SAECs) have recently attracted tremendous research interest
due to their often remarkable catalytic responses, unmatched by conventional catalysts. The …

Molecular carbons: How far can we go?

MW Wang, W Fan, X Li, Y Liu, Z Li, W Jiang, J Wu… - Acs Nano, 2023 - ACS Publications
The creation and development of carbon nanomaterials promoted material science
significantly. Bottom-up synthesis has emerged as an efficient strategy to synthesize …

Observation of fractional edge excitations in nanographene spin chains

S Mishra, G Catarina, F Wu, R Ortiz, D Jacob, K Eimre… - Nature, 2021 - nature.com
Fractionalization is a phenomenon in which strong interactions in a quantum system drive
the emergence of excitations with quantum numbers that are absent in the building blocks …

Topological frustration induces unconventional magnetism in a nanographene

S Mishra, D Beyer, K Eimre, S Kezilebieke… - Nature …, 2020 - nature.com
The chemical versatility of carbon imparts manifold properties to organic compounds, where
magnetism remains one of the most desirable but elusive. Polycyclic aromatic hydrocarbons …

Open-shell graphene fragments

W Zeng, J Wu - Chem, 2021 - cell.com
The electronic properties of finite-sized graphene fragments are strongly dependent on their
topological structures. The existence of two or more extended zigzag edges could lead to …

Synthetic Tailoring of graphene nanostructures with zigzag‐edged topologies: progress and perspectives

J Liu, X Feng - Angewandte Chemie International Edition, 2020 - Wiley Online Library
Experimental and theoretical investigations have revealed that the chemical and physical
properties of graphene are crucially determined by their topological structures. Therefore …

Orbital-symmetry effects on magnetic exchange in open-shell nanographenes

Q Du, X Su, Y Liu, Y Jiang, C Li, KK Yan, R Ortiz… - Nature …, 2023 - nature.com
Open-shell nanographenes appear as promising candidates for future applications in
spintronics and quantum technologies. A critical aspect to realize this potential is to design …

Uncovering the triplet ground state of triangular graphene nanoflakes engineered with atomic precision on a metal surface

J Li, S Sanz, J Castro-Esteban, M Vilas-Varela… - Physical Review Letters, 2020 - APS
Graphene can develop large magnetic moments in custom-crafted open-shell
nanostructures such as triangulene, a triangular piece of graphene with zigzag edges …

Collective all‐carbon magnetism in triangulene dimers

S Mishra, D Beyer, K Eimre, R Ortiz… - Angewandte …, 2020 - Wiley Online Library
Triangular zigzag nanographenes, such as triangulene and its π‐extended homologues,
have received widespread attention as organic nanomagnets for molecular spintronics, and …

On‐surface synthesis and collective spin excitations of a triangulene‐based nanostar

J Hieulle, S Castro, N Friedrich… - Angewandte Chemie …, 2021 - Wiley Online Library
Triangulene nanographenes are open‐shell molecules with predicted high spin state due to
the frustration of their conjugated network. Their long‐sought synthesis became recently …