Understanding polaritonic chemistry from ab initio quantum electrodynamics

M Ruggenthaler, D Sidler, A Rubio - Chemical Reviews, 2023 - ACS Publications
In this review, we present the theoretical foundations and first-principles frameworks to
describe quantum matter within quantum electrodynamics (QED) in the low-energy regime …

Single organic molecules for photonic quantum technologies

C Toninelli, I Gerhardt, AS Clark, A Reserbat-Plantey… - Nature Materials, 2021 - nature.com
Isolating single molecules in the solid state has allowed fundamental experiments in basic
and applied sciences. When cooled down to liquid helium temperature, certain molecules …

Cooperative quantum phenomena in light-matter platforms

M Reitz, C Sommer, C Genes - PRX Quantum, 2022 - APS
Quantum cooperativity is evident in light-matter platforms where quantum-emitter ensembles
are interfaced with confined optical modes and are coupled via the ubiquitous …

Phonon-induced optical dephasing in single organic molecules

C Clear, RC Schofield, KD Major, J Iles-Smith… - Physical review …, 2020 - APS
We present a joint experiment-theory analysis of the temperature-dependent emission
spectra, zero-phonon linewidth, and second-order correlation function of light emitted from a …

Key role of chromophore-modified vibrational modes on thermal broadening of single-molecule spectra in disordered solids

AO Savostianov, IY Eremchev, T Plakhotnik… - Physical Review B, 2024 - APS
For decades, the thermal broadening of zero-phonon lines of single organic molecules
embedded in amorphous solids was associated with their weak electron-phonon coupling to …

Molecular polaritonics in dense mesoscopic disordered ensembles

C Sommer, M Reitz, F Mineo, C Genes - Physical Review Research, 2021 - APS
We study the dependence of the vacuum Rabi splitting (VRS) on frequency disorder,
vibrations, near-field effects, and density in molecular polaritonics. In the mesoscopic limit …

One-dimensional photonic wire as a single-photon source: Implications of cavity QED to a phonon bath of reduced dimensionality

J Ferreira Neto, M Bundgaard-Nielsen, N Gregersen… - Physical Review B, 2024 - APS
While the semiconductor quantum dot placed in a solid-state material allows for
deterministic emission of single photons, the photon indistinguishability is strongly …

Quantum dynamics of a Bose polaron in a -dimensional Bose-Einstein condensate

MM Khan, H Terças, JT Mendonça, J Wehr… - Physical Review A, 2021 - APS
We study the quantum motion of an impurity atom immersed in a Bose-Einstein condensate
in arbitrary dimensions. It was shown, for all dimensions, that the Bogoliubov excitations of …

Quantum Thermometry with Single Molecules in Nanoprobes

V Esteso, R Duquennoy, RC Ng, M Colautti… - PRX Quantum, 2023 - APS
An understanding of heat transport is relevant to develo** efficient strategies for thermal
management in areas of study such as microelectronics, as well as for fundamental science …

Impact of vibrational modes in the plasmonic Purcell effect of organic molecules

D Zhao, REF Silva, C Climent, J Feist… - ACS …, 2020 - ACS Publications
By means of quantum tensor network calculations, we investigate the large Purcell effect
experienced by an organic molecule placed in the vicinity of a plasmonic nanostructure. In …