Understanding polaritonic chemistry from ab initio quantum electrodynamics
In this review, we present the theoretical foundations and first-principles frameworks to
describe quantum matter within quantum electrodynamics (QED) in the low-energy regime …
describe quantum matter within quantum electrodynamics (QED) in the low-energy regime …
Single organic molecules for photonic quantum technologies
Isolating single molecules in the solid state has allowed fundamental experiments in basic
and applied sciences. When cooled down to liquid helium temperature, certain molecules …
and applied sciences. When cooled down to liquid helium temperature, certain molecules …
Cooperative quantum phenomena in light-matter platforms
Quantum cooperativity is evident in light-matter platforms where quantum-emitter ensembles
are interfaced with confined optical modes and are coupled via the ubiquitous …
are interfaced with confined optical modes and are coupled via the ubiquitous …
Phonon-induced optical dephasing in single organic molecules
We present a joint experiment-theory analysis of the temperature-dependent emission
spectra, zero-phonon linewidth, and second-order correlation function of light emitted from a …
spectra, zero-phonon linewidth, and second-order correlation function of light emitted from a …
Key role of chromophore-modified vibrational modes on thermal broadening of single-molecule spectra in disordered solids
For decades, the thermal broadening of zero-phonon lines of single organic molecules
embedded in amorphous solids was associated with their weak electron-phonon coupling to …
embedded in amorphous solids was associated with their weak electron-phonon coupling to …
Molecular polaritonics in dense mesoscopic disordered ensembles
We study the dependence of the vacuum Rabi splitting (VRS) on frequency disorder,
vibrations, near-field effects, and density in molecular polaritonics. In the mesoscopic limit …
vibrations, near-field effects, and density in molecular polaritonics. In the mesoscopic limit …
One-dimensional photonic wire as a single-photon source: Implications of cavity QED to a phonon bath of reduced dimensionality
While the semiconductor quantum dot placed in a solid-state material allows for
deterministic emission of single photons, the photon indistinguishability is strongly …
deterministic emission of single photons, the photon indistinguishability is strongly …
Quantum dynamics of a Bose polaron in a -dimensional Bose-Einstein condensate
We study the quantum motion of an impurity atom immersed in a Bose-Einstein condensate
in arbitrary dimensions. It was shown, for all dimensions, that the Bogoliubov excitations of …
in arbitrary dimensions. It was shown, for all dimensions, that the Bogoliubov excitations of …
Quantum Thermometry with Single Molecules in Nanoprobes
An understanding of heat transport is relevant to develo** efficient strategies for thermal
management in areas of study such as microelectronics, as well as for fundamental science …
management in areas of study such as microelectronics, as well as for fundamental science …
Impact of vibrational modes in the plasmonic Purcell effect of organic molecules
By means of quantum tensor network calculations, we investigate the large Purcell effect
experienced by an organic molecule placed in the vicinity of a plasmonic nanostructure. In …
experienced by an organic molecule placed in the vicinity of a plasmonic nanostructure. In …