The observation of coherent dynamics ensuing from the excitation of molecular systems by
femtosecond laser pulses is at the heart of femtochemistry. The time-dependent evolution of …

Multidimensional Vibrational Coherence Spectroscopy Page 1 Vol.:(0123456789) Topics in
Current Chemistry (2018) 376:35 https://doi.org/10.1007/s41061-018-0213-4 1 3 REVIEW …

We report controlled excitation of ground-state rotational wave packet by pulse-sha**
technique. The experiment is conducted in nitrogen (N 2) at room temperature and …

We demonstrate the feasibility of the time‐delayed femtosecond CARS (fs‐CARS) technique
in a dense gas environment. The experiments were performed on N2 molecules between …

Time-resolved coherent Raman spectroscopy (CRS) is a powerful non-linear optical
technique for quantitative, in-situ analysis of chemically reacting flows, offering unparalleled …

The analysis of nonlinear spectroscopy, widely used to study the dynamics and structures of
condensed-phase matter, typically employs a perturbative approach noticing the weak …

Probing the real time dynamics of a reacting molecule remains one of the central challenges
in chemistry. Here we show how the time-dependent wave function of an excited-state …

Two-dimensional (2D) vibronic correlation spectra of molecular dimers are calculated, taking
a single vibration in each monomer into account. Within the employed wave function …

Abstract Femtosecond coherent anti-Stokes Raman scattering (fsCARS) spectroscopy,
together with perturbation theory based numerical calculation, is employed to study OH …

Nonlinear spectroscopic signals in liquid solution were calculated without treating the field-
matter interaction in a perturbative manner. The calculation is based on the assumption that …