Multiscale CO2 Electrocatalysis to C2+ Products: Reaction Mechanisms, Catalyst Design, and Device Fabrication

T Yan, X Chen, L Kumari, J Lin, M Li, Q Fan… - Chemical …, 2023 - ACS Publications
Electrosynthesis of value-added chemicals, directly from CO2, could foster achievement of
carbon neutral through an alternative electrical approach to the energy-intensive …

Enrichment of reactants and intermediates for electrocatalytic CO 2 reduction

PP Yang, MR Gao - Chemical Society Reviews, 2023 - pubs.rsc.org
The electrocatalytic carbon dioxide reduction reaction (CO2RR) presents a sustainable
route to convert renewable electricity to value-added fuels and feedstocks in the form of …

Electrochemical C–N coupling of CO 2 and nitrogenous small molecules for the electrosynthesis of organonitrogen compounds

X Peng, L Zeng, D Wang, Z Liu, Y Li, Z Li… - Chemical Society …, 2023 - pubs.rsc.org
Electrochemical C–N coupling reactions based on abundant small molecules (such as CO2
and N2) have attracted increasing attention as a new “green synthetic strategy” for the …

Accelerating electrochemical CO2 reduction to multi-carbon products via asymmetric intermediate binding at confined nanointerfaces

J Zhang, C Guo, S Fang, X Zhao, L Li, H Jiang… - Nature …, 2023 - nature.com
Abstract Electrochemical CO2 reduction (CO2R) to ethylene and ethanol enables the long-
term storage of renewable electricity in valuable multi-carbon (C2+) chemicals. However …

In Situ Infrared Spectroscopic Evidence of Enhanced Electrochemical CO2 Reduction and C–C Coupling on Oxide-Derived Copper

EP Delmo, Y Wang, Y Song, S Zhu… - Journal of the …, 2024 - ACS Publications
The reaction mechanism of CO2 electroreduction on oxide-derived copper has not yet been
unraveled even though high C2+ Faradaic efficiencies are commonly observed on these …

Experimental evidence of distinct sites for CO2-to-CO and CO conversion on Cu in the electrochemical CO2 reduction reaction

W Gao, Y Xu, L Fu, X Chang, B Xu - Nature Catalysis, 2023 - nature.com
The electrochemical CO2 reduction reaction on Cu is widely believed to occur via two
consecutive and orthogonal reaction steps, that is, CO2-to-CO and CO-to-C2+, on the same …

C2+ Selectivity for CO2 Electroreduction on Oxidized Cu-Based Catalysts

H Li, Y Jiang, X Li, K Davey, Y Zheng… - Journal of the …, 2023 - ACS Publications
Design for highly selective catalysts for CO2 electroreduction to multicarbon (C2+) fuels is
pressing and important. There is, however, presently a poor understanding of selectivity …

Membrane Electrode Assembly for Electrocatalytic CO2 Reduction: Principle and Application

Z Zhang, X Huang, Z Chen, J Zhu… - Angewandte …, 2023 - Wiley Online Library
Electrocatalytic CO2 reduction reaction (CO2RR) in membrane electrode assembly (MEA)
systems is a promising technology. Gaseous CO2 can be directly transported to the cathode …

Surface hydroxide promotes CO2 electrolysis to ethylene in acidic conditions

Y Cao, Z Chen, P Li, A Ozden, P Ou, W Ni… - Nature …, 2023 - nature.com
Performing CO2 reduction in acidic conditions enables high single-pass CO2 conversion
efficiency. However, a faster kinetics of the hydrogen evolution reaction compared to CO2 …

Superiority of dual‐atom catalysts in electrocatalysis: one step further than single‐atom catalysts

R Li, D Wang - Advanced Energy Materials, 2022 - Wiley Online Library
In recent years, dual‐atom catalysts (DACs) have attracted extensive attention, as an
extension of single‐atom catalysts (SACs). Compared with SACs, DACs have higher metal …