Applying Classical, Ab Initio, and Machine-Learning Molecular Dynamics Simulations to the Liquid Electrolyte for Rechargeable Batteries

N Yao, X Chen, ZH Fu, Q Zhang - Chemical Reviews, 2022 - ACS Publications
Rechargeable batteries have become indispensable implements in our daily life and are
considered a promising technology to construct sustainable energy systems in the future …

A review of solid electrolyte interphase (SEI) and dendrite formation in lithium batteries

B Li, Y Chao, M Li, Y **ao, R Li, K Yang, X Cui… - Electrochemical Energy …, 2023 - Springer
Lithium-metal batteries with high energy/power densities have significant applications in
electronics, electric vehicles, and stationary power plants. However, the unstable lithium …

Ion transport kinetics in low‐temperature lithium metal batteries

A Hu, F Li, W Chen, T Lei, Y Li, Y Fan… - Advanced Energy …, 2022 - Wiley Online Library
The deployment of rechargeable batteries is crucial for the operation of advanced portable
electronics and electric vehicles under harsh environment. However, commercial lithium‐ion …

Review on modeling of the anode solid electrolyte interphase (SEI) for lithium-ion batteries

A Wang, S Kadam, H Li, S Shi, Y Qi - NPJ Computational materials, 2018 - nature.com
A passivation layer called the solid electrolyte interphase (SEI) is formed on electrode
surfaces from decomposition products of electrolytes. The SEI allows Li+ transport and …

Molecular dynamics simulations of ionic liquids and electrolytes using polarizable force fields

D Bedrov, JP Piquemal, O Borodin… - Chemical …, 2019 - ACS Publications
Many applications in chemistry, biology, and energy storage/conversion research rely on
molecular simulations to provide fundamental insight into structural and transport properties …

Anionic coordination manipulation of multilayer solvation structure electrolyte for high‐rate and low‐temperature lithium metal battery

N Sun, R Li, Y Zhao, H Zhang, J Chen… - Advanced energy …, 2022 - Wiley Online Library
Challenges from high‐energy‐density storage applications have boosted the pursuit of
designing high‐rate and low‐temperature lithium (Li) metal batteries (LMBs). Formulating …

Pushing the limit of molecular dynamics with ab initio accuracy to 100 million atoms with machine learning

W Jia, H Wang, M Chen, D Lu, L Lin… - … conference for high …, 2020 - ieeexplore.ieee.org
For 35 years, ab initio molecular dynamics (AIMD) has been the method of choice for
modeling complex atomistic phenomena from first principles. However, most AIMD …

Effect of the electric double layer (EDL) in multicomponent electrolyte reduction and solid electrolyte interphase (SEI) formation in lithium batteries

Q Wu, MT McDowell, Y Qi - Journal of the American Chemical …, 2023 - ACS Publications
Electrolytes, consisting of salts, solvents, and additives, must form a stable solid electrolyte
interphase (SEI) to ensure the performance and durability of lithium (Li)-ion batteries …

The influence of FEC on the solvation structure and reduction reaction of LiPF6/EC electrolytes and its implication for solid electrolyte interphase formation

T Hou, G Yang, NN Rajput, J Self, SW Park, J Nanda… - Nano Energy, 2019 - Elsevier
Fluoroethylene carbonate (FEC) has been proposed as an effective electrolyte additive that
enhances the stability and elasticity of the solid electrolyte interphase (SEI) of emerging Si …

The state of understanding of the lithium-ion-battery graphite solid electrolyte interphase (SEI) and its relationship to formation cycling

SJ An, J Li, C Daniel, D Mohanty, S Nagpure… - Carbon, 2016 - Elsevier
An in-depth historical and current review is presented on the science of lithium-ion battery
(LIB) solid electrolyte interphase (SEI) formation on the graphite anode, including structure …