Tailor‐Engineered 2D Cocatalysts: Harnessing Electron–Hole Redox Center of 2D g‐C3N4 Photocatalysts toward Solar‐to‐Chemical Conversion and …

GZS Ling, SF Ng, WJ Ong - Advanced Functional Materials, 2022 - Wiley Online Library
Sparked by natural photosynthesis, solar photocatalysis using metal‐free graphitic carbon
nitride (g‐C3N4) with appealing electronic structure has turned up as the most captivating …

Computational discovery of transition-metal complexes: from high-throughput screening to machine learning

A Nandy, C Duan, MG Taylor, F Liu, AH Steeves… - Chemical …, 2021 - ACS Publications
Transition-metal complexes are attractive targets for the design of catalysts and functional
materials. The behavior of the metal–organic bond, while very tunable for achieving target …

New strategies for direct methane-to-methanol conversion from active learning exploration of 16 million catalysts

A Nandy, C Duan, C Goffinet, HJ Kulik - Jacs Au, 2022 - ACS Publications
Despite decades of effort, no earth-abundant homogeneous catalysts have been discovered
that can selectively oxidize methane to methanol. We exploit active learning to …

Using Computational Chemistry to Reveal Nature's Blueprints for Single-Site Catalysis of C–H Activation

A Nandy, H Adamji, DW Kastner, V Vennelakanti… - ACS …, 2022 - ACS Publications
The challenge of activating inert C–H bonds motivates a study of catalysts that draws from
what can be accomplished by natural enzymes and translates these advantageous features …

Performance of the r2SCAN Functional in Transition Metal Oxides

S Swathilakshmi, R Devi… - Journal of chemical theory …, 2023 - ACS Publications
We assess the accuracy and computational efficiency of the recently developed meta-
generalized gradient approximation (metaGGA) functional, restored regularized strongly …

Activating γ-graphyne nanoribbons as bifunctional electrocatalysts toward oxygen reduction and hydrogen evolution reactions by edge termination and nitrogen …

Y Lv, B Kang, Y Yuan, G Chen, JY Lee - Chemical Engineering Journal, 2022 - Elsevier
Carbon-based metal free materials (CMFCs) as electrocatalysts have been a hot issue and
are receiving growing attention. In this paper, we applied intensive density functional theory …

Large data set-driven machine learning models for accurate prediction of the thermoelectric figure of merit

Y Li, J Zhang, K Zhang, M Zhao, K Hu… - ACS Applied Materials & …, 2022 - ACS Publications
The figure of merit (zT) is a key parameter to measure the performance of thermoelectric
materials. At present, the prediction of zT values via machine leaning has emerged as a …

Machine learning to tame divergent density functional approximations: a new path to consensus materials design principles

C Duan, S Chen, MG Taylor, F Liu, HJ Kulik - Chemical Science, 2021 - pubs.rsc.org
Virtual high-throughput screening (VHTS) with density functional theory (DFT) and machine-
learning (ML)-acceleration is essential in rapid materials discovery. By necessity, efficient …

Accelerating materials-space exploration for thermal insulators by map** materials properties via artificial intelligence

TAR Purcell, M Scheffler, LM Ghiringhelli… - npj computational …, 2023 - nature.com
Reliable artificial-intelligence models have the potential to accelerate the discovery of
materials with optimal properties for various applications, including superconductivity …

Detection of multi-reference character imbalances enables a transfer learning approach for virtual high throughput screening with coupled cluster accuracy at DFT cost

C Duan, DBK Chu, A Nandy, HJ Kulik - Chemical Science, 2022 - pubs.rsc.org
Appropriately identifying and treating molecules and materials with significant multi-
reference (MR) character is crucial for achieving high data fidelity in virtual high-throughput …