Dielectric screening meets optimally tuned density functionals

L Kronik, S Kümmel - Advanced Materials, 2018 - Wiley Online Library
A short overview of recent attempts at merging two independently developed methods is
presented. These are the optimal tuning of a range‐separated hybrid (OT‐RSH) functional …

Modeling absorption spectra of molecules in solution

TJ Zuehlsdorff, CM Isborn - International Journal of Quantum …, 2019 - Wiley Online Library
The presence of solvent tunes many properties of a molecule, such as its ground and
excited state geometry, dipole moment, excitation energy, and absorption spectrum …

Machine learning enables highly accurate predictions of photophysical properties of organic fluorescent materials: Emission wavelengths and quantum yields

CW Ju, H Bai, B Li, R Liu - Journal of Chemical Information and …, 2021 - ACS Publications
The development of functional organic fluorescent materials calls for fast and accurate
predictions of photophysical parameters for processes such as high-throughput virtual …

Poisoning density functional theory with benchmark sets of difficult systems

T Gould, SG Dale - Physical Chemistry Chemical Physics, 2022 - pubs.rsc.org
Large benchmark sets like GMTKN55 [Goerigk et al., Phys. Chem. Chem. Phys., 2017, 19,
32184] let us analyse the performance of density functional theory over a diverse range of …

Machine-learning screening of luminogens with aggregation-induced emission characteristics for fluorescence imaging

Y Zhang, M Fan, Z Xu, Y Jiang, H Ding, Z Li… - Journal of …, 2023 - Springer
Due to the excellent biocompatible physicochemical performance, luminogens with
aggregation-induced emission (AIEgens) characteristics have played a significant role in …

Unveiling the photophysical and excited state properties of multi-resonant OLED emitters using combined DFT and CCSD method

P Sivasakthi, PK Samanta - Physical Chemistry Chemical Physics, 2024 - pubs.rsc.org
Multi-resonance thermally-activated delayed fluorescence (MR-TADF) is predominantly
observed in organoboron heteroatom-embedded molecules, featuring enhanced …

Spatial decay and limits of quantum solute–solvent interactions

G Weng, A Pang, V Vlcek - The Journal of Physical Chemistry …, 2023 - ACS Publications
Molecular excitations in the liquid-phase environment are renormalized by the surrounding
solvent molecules. Herein, we employ the GW approximation to investigate the solvation …

Do water's electrons care about electrolytes?

MN Pohl, E Muchová, R Seidel, H Ali, Š Sršeň… - Chemical …, 2019 - pubs.rsc.org
Ions have a profound effect on the geometrical structure of liquid water and an aqueous
environment is known to change the electronic structure of ions. Here we combine …

Performance of TDDFT Vertical Excitation Energies of Core‐Substituted Naphthalene Diimides

AK Narsaria, JD Ruijter, TA Hamlin… - Journal of …, 2020 - Wiley Online Library
We have evaluated the performance of various density functionals, covering generalized
gradient approximation (GGA), global hybrid (GH) and range‐separated hybrid (RSH), using …

[HTML][HTML] Efficient treatment of molecular excitations in the liquid phase environment via stochastic many-body theory

G Weng, V Vlček - The Journal of Chemical Physics, 2021 - pubs.aip.org
Accurate predictions of charge excitation energies of molecules in the disordered
condensed phase are central to the chemical reactivity, stability, and optoelectronic …