Multiscale CO2 Electrocatalysis to C2+ Products: Reaction Mechanisms, Catalyst Design, and Device Fabrication

T Yan, X Chen, L Kumari, J Lin, M Li, Q Fan… - Chemical …, 2023 - ACS Publications
Electrosynthesis of value-added chemicals, directly from CO2, could foster achievement of
carbon neutral through an alternative electrical approach to the energy-intensive …

Electrochemical reduction of carbon dioxide to multicarbon (C 2+) products: challenges and perspectives

B Chang, H Pang, F Raziq, S Wang… - Energy & …, 2023 - pubs.rsc.org
Electrocatalytic CO2 reduction has been developed as a promising and attractive strategy to
achieve carbon neutrality for sustainable chemical production. Among various reduction …

Atomic-scale surface restructuring of copper electrodes under CO2 electroreduction conditions

R Amirbeigiarab, J Tian, A Herzog, C Qiu… - Nature Catalysis, 2023 - nature.com
Potentiodynamic methods that induce structural changes in Cu catalysts for the
electrochemical reduction of CO2 (CO2RR) have been identified as a promising strategy for …

Coverage-driven selectivity switch from ethylene to acetate in high-rate CO2/CO electrolysis

P Wei, D Gao, T Liu, H Li, J Sang, C Wang… - Nature …, 2023 - nature.com
Tuning catalyst microenvironments by electrolytes and organic modifications is effective in
improving CO2 electrolysis performance. An alternative way is to use mixed CO/CO2 feeds …

Improving CO2-to-C2+ Product Electroreduction Efficiency via Atomic Lanthanide Dopant-Induced Tensile-Strained CuOx Catalysts

J Feng, L Wu, S Liu, L Xu, X Song… - Journal of the …, 2023 - ACS Publications
Cu is a promising electrocatalyst in CO2 reduction reaction (CO2RR) to high-value C2+
products. However, as important C–C coupling active sites, the Cu+ species is usually …

Constrained C2 adsorbate orientation enables CO-to-acetate electroreduction

J **, J Wicks, Q Min, J Li, Y Hu, J Ma, Y Wang, Z Jiang… - Nature, 2023 - nature.com
The carbon dioxide and carbon monoxide electroreduction reactions, when powered using
low-carbon electricity, offer pathways to the decarbonization of chemical manufacture …

Surface hydroxide promotes CO2 electrolysis to ethylene in acidic conditions

Y Cao, Z Chen, P Li, A Ozden, P Ou, W Ni… - Nature …, 2023 - nature.com
Performing CO2 reduction in acidic conditions enables high single-pass CO2 conversion
efficiency. However, a faster kinetics of the hydrogen evolution reaction compared to CO2 …

Imidazolium-functionalized Mo3P nanoparticles with an ionomer coating for electrocatalytic reduction of CO2 to propane

M Esmaeilirad, Z Jiang, AM Harzandi, A Kondori… - Nature Energy, 2023 - nature.com
Propane is a tri-carbon (C3) alkane widely used as a fuel. Despite recent advances in CO2
electrocatalysis, the production of C3+ molecules directly from CO2 is challenging due to …

Modulating electric field distribution by alkali cations for CO2 electroreduction in strongly acidic medium

J Gu, S Liu, W Ni, W Ren, S Haussener, X Hu - Nature Catalysis, 2022 - nature.com
The reaction of carbon dioxide with hydroxide to form carbonate in near-neutral or alkaline
medium severely limits the energy and carbon efficiency of CO2 electroreduction. Here we …

2022 roadmap on low temperature electrochemical CO2 reduction

IEL Stephens, K Chan, A Bagger… - Journal of Physics …, 2022 - iopscience.iop.org
Abstract Electrochemical CO 2 reduction (CO 2 R) is an attractive option for storing
renewable electricity and for the sustainable production of valuable chemicals and fuels. In …