Aromaticity of the planar hetero [8] circulenes and their doubly charged ions: NICS and GIMIC characterization

GV Baryshnikov, RR Valiev, NN Karaush… - Physical Chemistry …, 2014 - pubs.rsc.org
A series of planar hetero [8] circulenes and their doubly charged ions are studied by the
NICS and GIMIC methods to interpret the aromatic properties of these high symmetry …

First study of the thermal and storage stability of arenediazonium triflates comparing to 4-nitrobenzenediazonium tosylate and tetrafluoroborate by calorimetric …

AA Bondarev, EV Naumov, AZ Kassanova… - … Process Research & …, 2019 - ACS Publications
Herein, for the first time, using isothermal flow calorimetry and differential scanning
calorimetry (DSC)/thermal gravimetric analysis (TGA), we have determined the thermal …

Phenyl cation: A versatile intermediate

V Dichiarante, S Protti, M Fagnoni - Journal of Photochemistry and …, 2017 - Elsevier
Phenyl cations are short-lived electrophiles and can be smoothly generated by photolysis of
aromatic halides (chlorides, fluorides) and esters (sulfonates, sulfates and phosphates) in …

Impact sensitivity of aryl diazonium chlorides: Limitations of molecular and solid-state approach

SV Bondarchuk - Journal of Molecular Graphics and Modelling, 2019 - Elsevier
The mechanism of the compression-induced decomposition of aryl diazonium chlorides is
proposed on the basis of quantum-chemical calculations of both the isolated cations and …

State-dependent global and local electrophilicity of the aryl cations

SV Bondarchuk, BF Minaev - The Journal of Physical Chemistry A, 2014 - ACS Publications
Two alternative approaches vertical and adiabatic are used to estimate global and local
electrophilicity (ω and ω k+) indexes for a series of aryl cations in both the ground and first …

Thermally accessible triplet state of π-nucleophiles does exist. Evidence from first principles study of ethylene interaction with copper species

SV Bondarchuk, BF Minaev - RSC Advances, 2015 - pubs.rsc.org
Three different models of ethylene interaction with copper species, namely, the Cu (100)
surface, odd-numbered copper clusters C2H4/Cun (where n= 3, 7, 11, 15, 17, 19, 21, 25 and …

The singlet–triplet energy splitting of π-nucleophiles as a measure of their reaction rate with electrophilic partners

SV Bondarchuk, BF Minaev - Chemical Physics Letters, 2014 - Elsevier
The recently introduced nucleophilicity index (N) of unsaturated compounds, which are
typical π-nucleophiles, correlates (R= 0.9229) with their singlet–triplet energy splitting (Δ S …

Carbocations

RA McClelland - … 2011: An annual survey covering the …, 2014 - Wiley Online Library
Due to the extremely weak nucleophilicity of the carborane anion, carborane acids protonate
organic compounds, providing stable carbocation salts. This chapter begins with …

Methoxy-Substituted α,n-Didehydrotoluenes. Photochemical Generation and Polar vs Diradical Reactivity

C Raviola, D Ravelli, S Protti… - Journal of the American …, 2014 - ACS Publications
The photoreactivity of differently substituted (chloromethoxybenzyl) trimethylsilanes in
alcohols and alcohol/water mixtures has been investigated by means of a combined …

Theoretical study of the triplet state aryl cations recombination: A possible route to unusually stable doubly charged biphenyl cations

SV Bondarchuk, BF Minaev… - International Journal of …, 2013 - Wiley Online Library
The self‐recombination reactions of 4‐aminophenyl cations and parent phenyl cations, each
in ground triplet states, are studied within the framework of density functional theory. Only …