Coordinatively unsaturated metal sites (open metal sites) in metal–organic frameworks: design and applications

Ü Kökçam-Demir, A Goldman, L Esrafili… - Chemical Society …, 2020 - pubs.rsc.org
Metal–organic frameworks (MOFs) can contain open metal sites (OMS) or coordinatively
unsaturated sites (CUS) or open coordination sites (OCS) when vacant Lewis acid sites on …

Generating catalytic sites in UiO-66 through defect engineering

X Feng, HS Jena, C Krishnaraj, K Leus… - … Applied Materials & …, 2021 - ACS Publications
UiO-66 is regarded as an epitome of metal–organic frameworks (MOFs) because of its
stability. Defect engineering has been used as a toolbox to alter the performance of MOFs …

Boosting toluene oxidation by the regulation of Pd species on UiO-66: Synergistic effect of Pd species

X Zhang, F Bi, Z Zhao, Y Yang, Y Li, L Song, N Liu… - Journal of …, 2022 - Elsevier
Supported single-atoms and sub-nanometre clusters have exhibited superb catalytic
performance toward many reactions. However, inactivation of single-atom or cluster …

From fundamentals to applications: a toolbox for robust and multifunctional MOF materials

A Kirchon, L Feng, HF Drake, EA Joseph… - Chemical Society …, 2018 - pubs.rsc.org
In recent years, metal–organic frameworks (MOFs) have been regarded as one of the most
important classes of materials. The combination of various metal clusters and ligands …

A decade of UiO-66 research: a historic review of dynamic structure, synthesis mechanisms, and characterization techniques of an archetypal metal–organic …

J Winarta, B Shan, SM Mcintyre, L Ye… - Crystal Growth & …, 2019 - ACS Publications
UiO-66 is an archetypal metal–organic framework (MOF) with a very high surface area as
well as high thermal stability. It is found that the stability can be attributed to the metal oxide …

Imaging defects and their evolution in a metal–organic framework at sub-unit-cell resolution

L Liu, Z Chen, J Wang, D Zhang, Y Zhu, S Ling… - Nature …, 2019 - nature.com
Defect engineering of metal–organic frameworks (MOFs) offers promising opportunities for
tailoring their properties to specific functions and applications. However, determining the …

Electronic structure modeling of metal–organic frameworks

JL Mancuso, AM Mroz, KN Le, CH Hendon - Chemical reviews, 2020 - ACS Publications
Owing to their molecular building blocks, yet highly crystalline nature, metal–organic
frameworks (MOFs) sit at the interface between molecule and material. Their diverse …

Metal–organic and covalent organic frameworks as single-site catalysts

SMJ Rogge, A Bavykina, J Hajek, H Garcia… - Chemical Society …, 2017 - pubs.rsc.org
Heterogeneous single-site catalysts consist of isolated, well-defined, active sites that are
spatially separated in a given solid and, ideally, structurally identical. In this review, the …

Surface-supported metal–organic framework thin films: fabrication methods, applications, and challenges

J Liu, C Wöll - Chemical Society Reviews, 2017 - pubs.rsc.org
Surface-supported metal–organic framework thin films are receiving increasing attention as
a novel form of nanotechnology. New deposition techniques that enable the control of the …

Defect engineering: tuning the porosity and composition of the metal–organic framework UiO-66 via modulated synthesis

GC Shearer, S Chavan, S Bordiga, S Svelle… - Chemistry of …, 2016 - ACS Publications
Presented in this paper is a deep investigation into the defect chemistry of UiO-66 when
synthesized in the presence of monocarboxylic acid modulators under the most commonly …